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Generation of bright phase-matched circularly-polarized extreme ultraviolet high harmonics

机译:产生亮相匹配的圆偏振极紫外高谐波

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Circularly-polarized extreme ultraviolet and X-ray radiation is useful for analysing the structural, electronic and magnetic properties of materials. To date, such radiation has only been available at large-scale X-ray facilities such as synchrotrons. Here, we demonstrate the first bright, phase-matched, extreme ultraviolet circularly-polarized high harmonics source. The harmonics are emitted when bi-chromatic counter-rotating circularly-polarized laser pulses field-ionize a gas in a hollow-core waveguide. We use this new light source for magnetic circular dichroism measurements at the M-shell absorption edges of Co. We show that phase-matching of circularly-polarized harmonics is unique and robust, producing a photon flux comparable to linearly polarized high harmonic sources. This work represents a critical advance towards the development of table-top systems for element-specific imaging and spectroscopy of multiple elements simultaneously in magnetic and other chiral media with very high spatial and temporal resolution.
机译:圆极化的极紫外和X射线辐射可用于分析材料的结构,电子和磁性。迄今为止,这种辐射仅在同步辐射器等大型X射线设施中可用。在这里,我们演示了第一个明亮的,相位匹配的,极紫外圆偏振的高谐波源。当双色反向旋转的圆偏振激光脉冲将空心波导中的气体电离时,会发出谐波。我们将此新光源用于Co的M壳吸收边缘处的磁性圆二色性测量。我们证明,圆极化谐波的相位匹配是唯一且稳定的,产生的光子通量可与线性极化高谐波源相媲美。这项工作代表了开发台式系统的关键进展,该台式系统用于同时在磁性和其他手性介质中以很高的时空分辨率对多个元素进行元素特定的成像和光谱分析。

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