Rh(l)-catalyzed cleavage of unactivated C-O bonds - Carbonylative rearrangement reactions of allenyl ethers to 2-carboalkoxy-1,3-dienes

Paul A.Wender; Nicole M.Deschamps; Robert Sun

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Rh(l)-catalyzed cleavage of unactivated C-O bonds - Carbonylative rearrangement reactions of allenyl ethers to 2-carboalkoxy-1,3-dienes

机译：Rh（l）催化的未活化C-O键裂解-烯基醚向2-carboalkoxy-1,3-dienes的羰基化重排反应

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摘要

The initial examples of a Rh(I)-catalyzed carbonylative rearrangement reaction of allenyl ethers are described.The key reaction proceeds under remarkably mild conditions to provide good to excellent yields of 2-carboalkoxy-1,3-dienes.

机译：描述了Rh（I）催化的烯丙基醚羰基重排反应的初始实例。关键反应在非常温和的条件下进行，从而获得了2-羰基烷氧基-1,3-二烯的良好至优异的收率。

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《Canadian Journal of Chemistry》 |2005年第7期|共5页
作者
Paul A.Wender; Nicole M.Deschamps; Robert Sun;
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正文语种 eng
中图分类化学;
关键词
carbonylative rearrangement; C-O cleavage; sigma bond activation; rhodium catalysis; allenyl ethers;

机译：羰基重排;C-O裂解;σ键活化;铑催化;烯丙基醚;

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1. Rh(l)-catalyzed cleavage of unactivated C-O bonds - Carbonylative rearrangement reactions of allenyl ethers to 2-carboalkoxy-1,3-dienes [J] . Paul A.Wender, Nicole M.Deschamps, Robert Sun Canadian Journal of Chemistry . 2005,第6a7期

机译：Rh（l）催化的未活化C-O键裂解-烯基醚向2-carboalkoxy-1,3-dienes的羰基化重排反应
2. Reaction Pathways and Energetics of Etheric C-O Bond Cleavage Catalyzed by Lanthanide Triflates [J] . Rajeev S. Assary, Abdurrahman C. Atesin, Zhi Li ACS catalysis . 2013,第9期

机译：镧系元素三氟甲磺酸酯催化醚键C-O键断裂的反应途径和能量
3. Reaction Pathways and Energetics of Etheric C-O Bond Cleavage Catalyzed by Lanthanide Triflates [J] . Rajeev S. Assary, Abdurrahman C. Atesin, Zhi Li ACS catalysis . 2013,第9期

机译：镧系元素催化的反应途径和醚型C-O键切割的能量学
4. Nickel-Catalyzed Cross-Coupling Reaction of Anisole Derivatives with Organoboron Compounds via C-O Bond Cleavage [C] . Mamoru Tobisu, Toshiaki Shimasaki, Naoto Chatani Symposium on Organometallic Chemistry . 2008

机译：通过C-O键裂解镍催化偶氧衍生物与有机硼化合物的交叉偶联反应
5. Gold (I)-catalyzed Claisen rearrangement of allenyl vinyl ethers; A synthetic and mechanistic approach. [D] . Hallal, Kassem M. 2011

机译：金（I）催化的烯丙基乙烯基醚的克莱森重排；综合的和机械的方法。
6. Ring Opening Reactions through C-O Bond Cleavage Uniquely Adding Chemical Functionality to Boron Subphthalocyanine [O] . Catherine Bonnier, Timothy P. Bender 2015

机译：通过C-O键断裂的开环反应为硼亚酞菁硼独特地增加了化学官能度
7. NHeterocyclic Carbene-Catalyzed TruceSmiles Rearrangement of NArylacrylamides via the Cleavage of Unactivated C(aryl)N Bonds [O] . -1

机译：NORENCYCLIC CARBENE催化的结构通过未激活的C（芳基）N键的切割重新排列那酰胺酰胺

Rh(l)-catalyzed cleavage of unactivated C-O bonds - Carbonylative rearrangement reactions of allenyl ethers to 2-carboalkoxy-1,3-dienes

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