The ultraviolet photoelectron spectrum of the N-chlorothionylimide molecule (Cl-NSO) has been obtained and analyzed. The spectrum is interpreted by comparison with the known spectra of the parent compounds H-NSO, SO2and the related molecules Cl-NCO and H-NCO as well as with the aid ofab initioSCF-calculations in terms of ionization from the eight highest filled valence molecular orbitals in this molecule.
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