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Transient intraband absorption of light by semiconductor nanorods

机译:半导体纳米棒对光的瞬态带内吸收

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摘要

A unified approach based on the reduced-density-matrix formalism has been used to develop a theory of intraband energy absorption of probe pulses, induced by pump pulses in semiconductor nanorods in the shape of parallelipipeds or cylinders. The conditions are determined under which the dependence of the absorbed energy of the probe pulses on the delay time with respect to the pump pulses when intraband transitions occur is described by one or two exponential functions with exponents proportional to the energy-relaxation rates of the states of the electronic subsystem of the nanorods. It is shown that the transient spectroscopy of intraband absorption makes it possible to determine the relaxation rates of the energy of the electron states of the nanorods.
机译:基于降密度矩阵形式主义的统一方法已被用于发展探针脉冲的带内能量吸收理论,该理论由平行管道或圆柱体形状的半导体纳米棒中的泵浦脉冲诱导。确定在带内跃迁发生时,探针脉冲的吸收能量对相对于泵浦脉冲的延迟时间的依赖性由一个或两个指数函数描述,其指数与纳米棒电子子系统状态的能量弛豫率成正比。结果表明,带内吸收的瞬态光谱可以确定纳米棒电子态能量的弛豫率。

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