Copper/Iron-Cocatalyzed Highly Selective Tandem Reactions: Efficient Approaches to Z-γ-Alkylidene Lactones

Si Li; Wei Jia; Ning Jiao

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Copper/Iron-Cocatalyzed Highly Selective Tandem Reactions: Efficient Approaches to Z-γ-Alkylidene Lactones

机译：铜/铁共催化的高选择性串联反应：Z-γ-亚烷基内酯的有效方法

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摘要

Inexpensive copper/iron-cocatalyzed, efficient, highly regioselective and stereoselective one-pot tandem conjugate addition-cyclization-hydroly-sis-decarboxylation reactions have been developed, which provide efficient tandem reactions for C—C and C—O bond formation, and the novel synthetic methods of γ-alkylidenebutyrolactones.

机译：已经开发了廉价的铜/铁共催化，高效，高度区域选择性和立体选择性的一锅串联共轭加成-环化-水解-脱羧反应，为C-C和C-O键的形成提供了有效的串联反应， γ-亚烷基丁内酯的新颖合成方法。

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《Advanced synthesis & catalysis》 |2009年第4期|共7页
作者
Si Li; Wei Jia; Ning Jiao;
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正文语种 eng
中图分类物理化学（理论化学）、化学物理学;
关键词
copper; cyclization; hydrolysis; iron; lactones;

机译：铜;环化;水解;铁;内酯;

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专利

1. Copper/Iron-Cocatalyzed Highly Selective Tandem Reactions: Efficient Approaches to Z-γ-Alkylidene Lactones [J] . Si Li, Wei Jia, Ning Jiao Advanced synthesis & catalysis . 2009,第4期

机译：铜/铁共催化的高选择性串联反应：Z-γ-亚烷基内酯的有效方法
2. AgNO3 catalyzed cyclization of propargyl-Meldrum's acids in aqueous solvent: highly selective synthesis of Z-γ-alkylidene lactones [J] . Wei Jia, Si Li, Miao Yu Tetrahedron letters: The International Journal for the Rapid Publication of Preliminary Communications in Organic Chemistry . 2009,第38期

机译：AgNO3在水性溶剂中催化炔丙基-马德鲁姆酸的环化：Z-γ-亚烷基内酯的高度选择性合成
3. Ylide hydrolysis in tandem reactions: A highly Z/E-selective access to 3-alkylidene dihydrobenzofurans and related analogues [J] . Zhu J.-B., Wang P., Liao S., Organic letters . 2013,第12期

机译：串联反应中的叶立德水解：高度Z / E选择性获得3-亚烷基二氢苯并呋喃及相关类似物
4. Synthesis of Biologically Relevant Natural and Unnatural Gamraα-Lactones and Lactams via Tandem Allylboration/Cyclization Reactions [C] . Tim G. Elford, Dennis G. Hall European Symposium on Organic Chemistry . 2009

机译：通过串联烯丙基硼酸盐/环化反应合成生物相关天然和非自然GAMRAα-内酯和内酰胺的方法
5. I. Zinc-mediated homologation-cyclopropanation in beta-diketones and selectivity within cyclopropanoxide rearrangements. II. Zinc-mediated tandem chain extension-aldol reaction and formation of substituted gamma-lactones. [D] . Bala, Kaushik. 2016

机译：I.锌介导的β-二酮中的同源-环丙烷化和环丙烷氧化物重排内的选择性。二。锌介导的串联扩链-醛醇缩合反应和取代的γ-内酯的形成。
6. Efficient and Selective Formation of Macrocyclic Disubstituted Z Alkenes by Ring-Closing Metathesis (RCM) Reactions Catalyzed by Mo- or W-Based Monoaryloxide Pyrrolide (MAP) Complexes. Applications to Total Syntheses of Epilachnene Yuzu Lactone Ambrettolide Epothilone C and Nakadomarin A [O] . Chenbo Wang, Miao Yu, Andrew F. Kyle, -1

机译：通过大环二取代烯烃Ž的高效和选择性形成闭环由钼或钨为基础的monoaryloxide吡咯（map）配合物催化复分解反应（RCm）反应。应用Epilachnene的全合成柚子内酯黄葵内酯埃博霉素C和那卡多莫林一
7. Highly selective and efficient photocatalytic reduction of nitrate in water by a tandem reaction system consisting of Pt/TiO 2 and SnPd/Al 2 O 3 : A comparative study of the tandem reaction system with a typical semiconductor photocatalyst, SnPd/TiO 2 [O] . Jun Hirayama, Yuichi Kamiya 2017

机译：由Pt / TiO 2和SnPD / Al 2 O 3组成的串联反应系统在水中具有高度选择性和高效的光催化还原硝酸盐：典型半导体光催化剂的串联反应系统的比较研究，SNPD / TiO 2

Copper/Iron-Cocatalyzed Highly Selective Tandem Reactions: Efficient Approaches to Z-γ-Alkylidene Lactones

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