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首页> 外文期刊>International Journal of Environmental Impacts: Management, Mitigation and Recovery >CHEMICAL CHARACTERISTICS OF WATER-SOLUBLE IONS AND METAL ELEMENTS IN AMBIENT PARTICLES OF SAITAMA, JAPAN DURING THE SPRING ASIAN DUST EVENT, 2017
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CHEMICAL CHARACTERISTICS OF WATER-SOLUBLE IONS AND METAL ELEMENTS IN AMBIENT PARTICLES OF SAITAMA, JAPAN DURING THE SPRING ASIAN DUST EVENT, 2017

机译:水溶性离子的化学特征金属元素在埼玉县环境粒子,日本在春季亚洲沙尘事件,2017年

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Metropolitan Tokyo area in Japan suffered from a strong Asian dust event which was lasted for 3 days from May 6 to May 8 in 2017. Asian dust particles are usually originated from the deserts of Mongolia and Kazakhstan and could be absorbed air pollutants contained the metals, water-soluble and organic matters during transport process. In this research, two sampling sites called 10F (30 m height above ground level) and roadside in Saitama were selected to collect five different size particles (PM_(1.1), PM_(1.1-2.0), PM_(2.0-3.3), PM_(3.3-7.0) and the coarse particles (>7.0 μm) of three different events: (1) before Asian dust event (B.A.), (2) during Asian dust event (D.A.) and (3) after Asian dust event (A.A.). Eight water-soluble ionic and 23 elemental species in D.A. event were higher than other periods. In D.A. event, the ionic contents in 10F were high to 10.3 μg/m~3 and the elemental contents in roadside were 6.50 μg/m~3 which were higher than those in roadside. Ionic contents were mainly distributed in PM_(1.1) with the high contents of secondary particles (NH_4~+, NO_3~- and SO_4~(2-)). Ca~(2+), Cl~- and Na~+ were more enriched in the coarse particles. Ion balance in D.A. event was more basic in 10F and more acidic in roadside. The higher ratios of NO_3~-/SO_4~(2-) in PM_(1.1) were also occurred in D.A. event. Total elements were high (6,050 ng/m~3) in 10F with the several times increasing in PM_(3.3-7.0) and the coarse particles, and the great contribution form the crustal elements (Al, Fe, Na, Mg and K). Enrichment factors (EFs) of trace elements in PM_(1.1) indicating the anthropogenic sources might be the main sources of those ions. EFs in the coarse particles indicating high concentrations of crustal elements might be affected by the Asian dust event. The analysis of air masses backward trajectories showed that the deserts of Mongolia and Kazakhstan and the northern part of China were the important air pollutant origins in Asian dust events with long-distance transport.
机译:大都会在日本东京地区遭受强劲的亚洲沙尘事件持续了3天从5月6日到2017年5月8日。粒子通常起源于沙漠蒙古和哈萨克斯坦和吸收空气污染物中含有金属,水溶性和有机物运输过程。网站叫10 f(高出地面30米高度)在埼玉县和路边被选来收集五个不同大小粒子(PM_ (1.1),PM_ (1.1 - -2.0), PM_ (2.0 - -3.3), PM_ (3.3 - -7.0)粗颗粒(> 7.0μm)三种不同事件:(1)前亚洲沙尘事件(学士),(2)在亚洲沙尘事件后(D.A.)和(3)亚洲沙尘事件(大家)。离子和23种元素在D.A.事件高于其他时期。离子含量高10 f 10.3μg / m ~ 3和路边的基本内容是6.50μg / m ~ 3高于那些在路边。离子主要分布在内容PM_(1.1)与高中学的内容粒子(NH_4 ~ +, NO_3 ~ -和SO_4 ~(2 -))。Ca ~ (2 +), Cl ~ -和Na ~ +更丰富的粗颗粒。更基本的在路边10 f和酸性更强。比率越高的NO_3 ~ - / SO_4 ~ (2 -) PM_ (1.1)也发生在D.A.事件。高(6050 ng / m ~ 3) 10 f数次增加PM_(3.3 - -7.0)和粗糙粒子,形成了伟大的贡献地壳元素(铝、铁、钠、镁和K)。微量元素的富集因素(EFs)PM_(1.1)表明人为来源可能这些离子的主要来源。粗颗粒表明高地壳元素的浓度受到亚洲沙尘事件的影响。空气质量逆向轨迹显示沙漠的蒙古和哈萨克斯坦和中国北部重要的空气污染物起源于亚洲沙尘事件长途运输。

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