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Strain engineering of optical properties in transparent VO2/muscovite heterostructures dagger double dagger

机译:透明VO2 / Muscovite的光学性能应变工程异性结构匕首双匕首

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Transparent VO2/muscovite heterostructures have attracted considerable attention because of their unique chemical and physical properties and potential practical applications. In this paper, we investigated the influence of uniaxial mechanical strain on the optical properties of VO2/muscovite heterostructures through Raman scattering and optical transmittance measurements. Under applied strain, linear shifts in peak positions of Raman-active phonon modes at approximately 340, 309, and 391 cm(-1) were observed. The extracted Gruneisen parameter values were approximately between 0.44 and 0.57. Furthermore, a pronounced strain-induced change in the metal-insulator transition (MIT) temperature was observed, which decreased under compressive strain and increased under tensile strain. The rates of MIT temperature variation reached 4.5 degrees C per % and 7.1 degrees C per % at a wavelength of 1200 nm during heating and cooling processes, respectively. These results demonstrate that the modulation of the optical properties of VO2/muscovite heterostructures is controllable and reversible through strain engineering, opening up new opportunities for applications in flexible and tunable photonic devices.
机译:透明VO2/白云母异质结构因其独特的化学和物理性质以及潜在的实际应用而受到广泛关注。在本文中,我们通过拉曼散射和光学透射测量研究了单轴机械应变对VO2/白云母异质结构光学性质的影响。在外加应变下,在大约340、309和391厘米(-1)处观察到拉曼有源声子模的峰值位置发生线性位移。提取的Gruneisen参数值大约在0.44和0.57之间。此外,观察到金属-绝缘体转变(MIT)温度的显著应变诱导变化,在压缩应变下降低,在拉伸应变下增加。在加热和冷却过程中,MIT在1200 nm波长下的温度变化率分别达到4.5摄氏度/%和7.1摄氏度/%。这些结果表明,通过应变工程,VO2/白云母异质结构的光学性质的调制是可控和可逆的,为在柔性和可调谐光子器件中的应用开辟了新的机会。

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