Self‐Assembly of MXene‐Surfactants at Liquid–Liquid Interfaces: From Structured Liquids to 3D Aerogels

Shi Shaowei; Qian Bingqing; Wu Xinyu; Sun Huilou; Wang Haiqiao; Zhang Hao‐Bin; Yu Zhong‐Zhen; Russell Thomas P.

摘要

Abstract >2D transition metal carbides and nitrides (MXenes), a class of emerging nanomaterials with intriguing properties, have attracted significant attention in recent years. However, owing to the highly hydrophilic nature of MXene nanosheets, assembly strategies of MXene at liquid–liquid interfaces have been very limited and challenging. Herein, through the cooperative assembly of MXene and amine‐functionalized polyhedral oligomeric silsesquioxane at the oil–water interface, we report the formation, assembly, and jamming of a new type MXene‐based Janus‐like nanoparticle surfactants, termed MXene‐surfactants (MXSs), which can significantly enhance the interfacial activity of MXene nanosheets. More importantly, this simple assembly strategy opens a new platform for the fabrication of functional MXene assemblies from mesoscale (e.g., structured liquids) to macroscale (e.g., aerogels), that can be used for a range of applications, including nanocomposites, electronic devices, and all‐liquid microfluidic devices. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> <P> 2D过渡金属碳化物和氮化物（MxENES），近年来引起了一类具有有趣性质的新出现的纳米材料。然而，由于MXENE NANOSHESS的高亲水性，液 - 液界面在液态 - 液体界面的组装策略非常有限和具有挑战性。在此，通过油水界面的MXENE和胺官能化多面体镁硅氧烷的协同组装，我们报告了新型MXENE的Janus样纳米颗粒表面活性剂的形成，组装和干扰，称为MxENE-表面活性剂（MXS）），它可以显着增强MxEne NanosheS的界面活性。更重要的是，这种简单的装配策略为从Mescroscale（例如，结构化液体）制造到宏观（例如，Aerogels）的功能MxENE组件制造的新平台，其可用于一系列应用，包括纳米复合材料，电子设备，和全液体微流体装置。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2019年第50期</span><b style="margin: 0 2px;">|</b><span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Shi Shaowei&option=202" target="_blank" rel="nofollow">Shi Shaowei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Qian Bingqing&option=202" target="_blank" rel="nofollow">Qian Bingqing;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wu Xinyu&option=202" target="_blank" rel="nofollow">Wu Xinyu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sun Huilou&option=202" target="_blank" rel="nofollow">Sun Huilou;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Haiqiao&option=202" target="_blank" rel="nofollow">Wang Haiqiao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Hao‐Bin&option=202" target="_blank" rel="nofollow">Zhang Hao‐Bin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yu Zhong‐Zhen&option=202" target="_blank" rel="nofollow">Yu Zhong‐Zhen;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Russell Thomas P.&option=202" target="_blank" rel="nofollow">Russell Thomas P.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Beijing Advanced Innovation Center for Soft Matter Science and EngineeringBeijing University of Chemical TechnologyBeijing 100029 China;</p> <p>Beijing Advanced Innovation Center for Soft Matter Science and EngineeringBeijing University of Chemical TechnologyBeijing 100029 China;</p> <p>State Key Laboratory of Organic-Inorganic CompositesBeijing University of Chemical TechnologyBeijing 100029 China;</p> <p>Beijing Advanced Innovation Center for Soft Matter Science and EngineeringBeijing University of Chemical TechnologyBeijing 100029 China;</p> <p>State Key Laboratory of Organic-Inorganic CompositesBeijing University of Chemical TechnologyBeijing 100029 China;</p> <p>State Key Laboratory of Organic-Inorganic CompositesBeijing University of Chemical TechnologyBeijing 100029 China;</p> <p>State Key Laboratory of Organic-Inorganic CompositesBeijing University of Chemical TechnologyBeijing 100029 China;</p> <p>Beijing Advanced Innovation Center for Soft Matter Science and EngineeringBeijing University of Chemical TechnologyBeijing 100029 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=aerogels&option=203" rel="nofollow">aerogels;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=interfacial assembly&option=203" rel="nofollow">interfacial assembly;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=jamming&option=203" rel="nofollow">jamming;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=MXene surfactants&option=203" rel="nofollow">MXene surfactants;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=structured liquids&option=203" rel="nofollow">structured liquids;</a> </p> <div class="translation"> 机译：Aerogels;界面组装;干扰;mxene表面活性剂;结构液体; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704028163766.html">Self‐Assembly of MXene‐Surfactants at Liquid–Liquid Interfaces: From Structured Liquids to 3D Aerogels</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Shi Shaowei&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Shi Shaowei,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Qian Bingqing&option=202" 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href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=杨明&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,杨明</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=堵雷&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,堵雷</a> <span> <a href="/journal-cn-23550/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 武汉轻工大学学报 </a> </span> <span> . 2016</span><span>,第001期</span> </span> </div> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/academic-journal-cn_journal-zhengzhou-university-light-industry-natural-science-edition_thesis/020128346720.html">金纳米粒子在液/液界面自组装</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=陈志军&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 陈志军</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=杨清香&option=202" target="_blank" rel="nofollow" class="tuijian_auth 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