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Transforming Porous Organic Cages into Porous Ionic Liquids via a Supramolecular Complexation Strategy

机译：通过超分子络合策略将多孔有机笼转化为多孔离子液体

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Abstract > Porous liquids are a type of porous materials that engineer permanent porosity into unique flowing liquids, exhibiting promising functionalities for a variety of applications. Here a Type?I porous liquid is synthesized by transforming porous organic cages into porous ionic liquids via a supramolecular complexation strategy. Simple physical mixing of 18‐crown‐6 with task‐specific anionic porous organic cages affords a porous ionic liquid with anionic porous organic cages as the anionic parts and 18‐crown‐6/potassium ion complexes as the cationic parts. In contrast, mixing of 15‐crown‐5 and anionic porous organic cages in a 2:1 ratio gives only solids, while the addition of excess 15‐crown‐5 affords a Type?II porous liquid. The permanent porosity in the cage‐based porous liquids has been also confirmed by molecular simulation, positron (e + ) annihilation lifetime spectroscopy, and enhanced gas sorption capacity compared with pure crown ethers. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 多孔液体是一种多孔材料，即将永久性孔隙率成独特的流动液体，表现出各种应用的有希望的功能。这里通过超分子络合策略将多孔有机笼转化为多孔离子液体来合成一种类型的α。用任务特异性阴离子多孔有机笼的18冠-6的简单物理混合提供多孔离子液体，其具有阴离子多孔有机笼作为阴离子份和18-冠-6 /钾离子配合物作为阳离子份。相反，在2：1的比例中混合15-冠-5和阴离子多孔有机笼仅提供固体，同时添加过量的15冠-5提供αII多孔液体。笼子基多孔液中的永久性孔隙也通过分子模拟，正电子（E + </ sup> ）与纯冠醚相比，湮灭寿命光谱，增强的气体吸附能力。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第6期</span><b style="margin: 0 2px;">|</b><span>共5页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jie Kecheng&option=202" target="_blank" rel="nofollow">Jie Kecheng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Onishi Nicole&option=202" target="_blank" rel="nofollow">Onishi Nicole;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Schott Jennifer A.&option=202" target="_blank" rel="nofollow">Schott Jennifer A.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Popovs Ilja&option=202" target="_blank" rel="nofollow">Popovs Ilja;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jiang De‐en&option=202" target="_blank" rel="nofollow">Jiang De‐en;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Mahurin Shannon&option=202" target="_blank" rel="nofollow">Mahurin Shannon;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dai Sheng&option=202" target="_blank" rel="nofollow">Dai Sheng;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of ChemistryThe University of TennesseeKnoxville Tennessee 37996-1600 USA;</p> <p>Department of ChemistryUniversity of CaliforniaRiverside California 92521 USA;</p> <p>Department of ChemistryThe University of TennesseeKnoxville Tennessee 37996-1600 USA;</p> <p>Chemical Sciences DivisionOak Ridge National LaboratoryOak Ridge Tennessee 37831-6201 USA;</p> <p>Department of ChemistryUniversity of CaliforniaRiverside California 92521 USA;</p> <p>Chemical Sciences DivisionOak Ridge National LaboratoryOak Ridge Tennessee 37831-6201 USA;</p> <p>Department of ChemistryThe University of TennesseeKnoxville Tennessee 37996-1600 USA;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=crown ethers&option=203" rel="nofollow">crown ethers;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=ionic liquids&option=203" rel="nofollow">ionic liquids;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=microporous materials&option=203" rel="nofollow">microporous materials;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=porous liquids&option=203" rel="nofollow">porous liquids;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=porous organic cages&option=203" rel="nofollow">porous organic cages;</a> </p> <div class="translation"> 机译：皇冠醚;离子液体;微孔材料;多孔液体;多孔有机笼; 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