Electron transfer kinetics of methylviologen included in 4-sulfonatocalix[n]arenes at glassy carbon electrode; adiabaticity and activation energy

Yuki Takahashi; Takashi Fujihara; Naritaka Kobayashi; Seiichiro Nakabayashi; Zsombor Miskolczy; László Biczók

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Electron transfer kinetics of methylviologen included in 4-sulfonatocalix[n]arenes at glassy carbon electrode; adiabaticity and activation energy

机译：在玻璃碳电极中包含4-磺酰肽[n]中包含的电子转移动力学。绝热与激活能量

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Quasi-reversible single electron transfer (ET) kinetics of methylviologen partly-included at the rim of 4-sulfonatocalix[n]arenes (n?=?4,6 and 8) has been investigated in aqueous solution. ET rates were measured by Nicholson method with relatively large potential scan rates (0.9?V/s?

机译：在水溶液中研究了甲基硫代甲基甲基甲基甲基甲基甲基甲基甲基的甲基硫代的甲基硫代的甲基硫代的动力学。 ET率通过尼科尔森方法测量，潜在扫描速率相对较大（0.9≤v/s≤≤≤≤≤≤50≤v/ s）。 ET在MV + / MV2 +和电极表面之间绝热地进行。在高速循环伏安法条件下，不建立激活状态下的宿主客人绑定平衡。非平衡稳定能量与空腔的大小无关。在不包含任何包含的情况下，ET的活化能量为70-80％。

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来源
《Chemical Physics Letters》 |2018年第2018期|共6页
作者
Yuki Takahashi; Takashi Fujihara; Naritaka Kobayashi; Seiichiro Nakabayashi; Zsombor Miskolczy; László Biczók;
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作者单位

Department of Chemistry Graduate School of Science and Engineering Saitama University;

Department of Chemistry Graduate School of Science and Engineering Saitama University;

Division of Strategic Research and Development Graduate School of Science and Engineering Saitama University;

Department of Chemistry Graduate School of Science and Engineering Saitama University;

Institute of Materials and Environmental Chemistry Research Centre for Natural Sciences Hungarian Academy of Sciences;

Institute of Materials and Environmental Chemistry Research Centre for Natural Sciences Hungarian Academy of Sciences;

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正文语种 eng
中图分类物理化学（理论化学）、化学物理学;
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1. Electron transfer kinetics of methylviologen included in 4-sulfonatocalix[n]arenes at glassy carbon electrode; adiabaticity and activation energy [J] . Yuki Takahashi, Takashi Fujihara, Naritaka Kobayashi, Chemical Physics Letters . 2018,第期

机译：在玻璃碳电极中包含4-磺酰肽[n]中包含的电子转移动力学。绝热与激活能量
2. Double-layer correction for electron-transfer kinetics at glassy carbon and mercury electrodes in N,N-dimethylformamide [J] . Meneses AB, Antonello S, Arevalo MC, Electroanalysis . 2006,第4期

机译：N，N-二甲基甲酰胺中玻璃碳和汞电极上电子转移动力学的双层校正
3. Control of catechol and hydroquinone electron-transfer kinetics on native and modified glassy carbon electrodes [J] . DuVall SH., McCreery RL. Analytical chemistry . 1999,第20期

机译：控制天然和修饰玻碳电极上邻苯二酚和对苯二酚的电子转移动力学
4. Facilitated electron transfer of dopamine, adrenaline and ascorbicacid at glassy carbon electrode by modification of a self-assembledbi-lipid film of 5, 5-ditetradecyl-2-(2-trimethyl-ammonioethyl)-1,3-dioxane bromide [C] . International Beijing conference and exhibition on instrumental analysis;BCEIA 2003 . 2003

机译：通过修饰5，5-二十四烷基-2-（2-三甲基-氨乙基）-1,3-二恶烷溴化物的自组装双脂质膜，促进多巴胺，肾上腺素和抗坏血酸在玻璃碳电极上的电子转移
5. Electron transfer kinetics of catechols on modified glassy carbon electrodes. [D] . DuVall, Stacy Hunt. 2000

机译：改性玻璃碳电极上邻苯二酚的电子转移动力学。
6. Direct Electron Transfer of Hemoglobin on Manganese III Oxide-Ag Nanofibers Modified Glassy Carbon Electrode [O] . Masoud Negahdary, Gholamreza Mazaheri, Somyyeh Rad, 2009

机译：血红蛋白在三氧化锰-Ag纳米纤维修饰的玻碳电极上的直接电子转移
7. Electron transfer kinetics of methylviologen included in 4-sulfonatocalixnarenes at glassy carbon electrode; adiabaticity and activation energy [O] . Yuki Takahashi, Takashi Fujihara, Naritaka Kobayashi, 2018

机译：在玻璃状碳电极中包含4-磺胺肽n中包含的电子转移动力学。绝热与激活能量
8. Fast Heterogeneous Electron Transfer Rates for Glassy Carbon Electrodes without Polishing or Activation Procedures [R] . Rice, R., Alfred, C., McCreery, R. 1989

机译：没有抛光或活化程序的玻碳电极的快速非均相电子转移率

Electron transfer kinetics of methylviologen included in 4-sulfonatocalix[n]arenes at glassy carbon electrode; adiabaticity and activation energy

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