Surface‐enhanced micro‐        <fc xmlns='http://www.wiley.com/namespaces/wiley'>CARS</fc>CARS        mapping of a nanostructured cerium dioxide/aluminum film surface with gold nanoparticle‐bound organic molecules

Fabelinsky Viktor I.; Kozlov Dimitrii N.; Orlov Sergey N.; Polivanov Yury N.; Shcherbakov Ivan A.; Smirnov Valery V.; Vereschagin Konstantin A.; Arzumanyan Grigory M.; Mamatkulov Kahramon Z.; Afanasiev Konstantin N.; Lagarkov Andrey N.; Ryzhikov Ilya A.; Sarychev Andrey K.; Budashov Igor A.; Nechaeva Natalia L.; Kurochkin Ilya N.

摘要

Abstract > Highly contrast epi‐surface‐enhanced coherent anti‐Stokes Raman scattering (SECARS) microimages of Au‐nanoparticle‐bound organic reporter molecule distributions at a surface of novel surface‐enhanced Raman scattering (SERS)‐active metamaterial junctions, based on nanoparticles spread over a nanostructured CeO <sub>2</sub> faceted dielectric film, deposited on an Al sublayer, were recorded at two‐color picosecond excitation of the surface in the near‐infrared spectral range. For this, a scanning confocal laser‐based micro‐CARS spectrometer was employed. The investigations showed that at Raman resonant laser excitation of the molecules/Au‐NP conjugates immobilized on the surface strong SECARS signals can be generated with laser powers not deteriorating the conjugates. Coupling CARS with the plasmonic metamaterial structures under investigation provided excellent chemical imaging contrast (up to 400) for biochemically relevant 5‐thio(2‐nitrobenzoic acid) and 4‐mercaptophenylboronic acid reporter molecules. Taking into account easy handling and utmost long‐term stability of the investigated metamaterial junction at ambient conditions, it might be considered as a promising perspective for a single‐molecule‐sensitivity surface‐enhanced Raman scattering or SECARS biosensor. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><abstract xmlns =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <title type =“main”>抽象</ title> >高度对比度基于纳米颗粒在纳米结构上扩散在新型表面增强拉曼散射（SERS） - 活性超材料结的表面的Au-naniparticle的有机报告分子分子的eu-nanimarticle-nanigational报告分子分子的显微散射（secars）微观散射CEO <sub> 2 </ sub>沉积在Al子层上的刻面式介电膜，在近红外光谱范围内的表面的两种颜色皮秒激励下记录。为此，采用了一种扫描共聚焦激光基微型汽车光谱仪。该研究表明，在拉曼共振激光激发的在固定在表面上的分子/ Au-NP缀合物，可以通过激光功率产生不劣化缀合物的激光功率产生。耦合车辆采用调查的等离子体超材料结构提供了优异的化学成像对比（最多400），用于生物化学相关的5-ZHIO（2-硝基苯甲酸）和4-巯基苯甲酸报道分子。考虑到环境条件下调查的超材料结的易于处理和最大的长期稳定性，可能被认为是对单分子敏感性表面增强拉曼散射或SECAR生物传感器的有希望的前景。 </ p> </ abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-35645/'>《Journal of Raman Spectroscopy: An International Journal for Original Work in All Aspects of Raman Spectroscopy, Including Higher Order Processes, and Also Brillouin- and Rayleigh Scattering》</a> <b style="margin: 0 2px;">|</b><span>2018年第7期</span><b style="margin: 0 2px;">|</b><span>共10页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Fabelinsky Viktor I.&option=202" target="_blank" rel="nofollow">Fabelinsky Viktor I.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kozlov Dimitrii N.&option=202" target="_blank" rel="nofollow">Kozlov Dimitrii N.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Orlov Sergey N.&option=202" target="_blank" rel="nofollow">Orlov Sergey N.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Polivanov Yury N.&option=202" target="_blank" rel="nofollow">Polivanov Yury N.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Shcherbakov Ivan A.&option=202" target="_blank" rel="nofollow">Shcherbakov Ivan A.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Smirnov Valery V.&option=202" target="_blank" rel="nofollow">Smirnov Valery V.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Vereschagin Konstantin A.&option=202" target="_blank" rel="nofollow">Vereschagin Konstantin A.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Arzumanyan Grigory M.&option=202" target="_blank" rel="nofollow">Arzumanyan Grigory M.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Mamatkulov Kahramon Z.&option=202" target="_blank" rel="nofollow">Mamatkulov Kahramon Z.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Afanasiev Konstantin N.&option=202" target="_blank" rel="nofollow">Afanasiev Konstantin N.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lagarkov Andrey N.&option=202" target="_blank" rel="nofollow">Lagarkov Andrey N.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ryzhikov Ilya A.&option=202" target="_blank" rel="nofollow">Ryzhikov Ilya A.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sarychev Andrey K.&option=202" target="_blank" rel="nofollow">Sarychev Andrey K.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Budashov Igor A.&option=202" target="_blank" rel="nofollow">Budashov Igor A.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Nechaeva Natalia L.&option=202" target="_blank" rel="nofollow">Nechaeva Natalia L.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kurochkin Ilya N.&option=202" target="_blank" rel="nofollow">Kurochkin Ilya N.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>A.M. Prokhorov General Physics InstituteRussian Academy of SciencesVavilov str. 38 119991 Moscow Russia;</p> <p>A.M. Prokhorov General Physics InstituteRussian Academy of SciencesVavilov str. 38 119991 Moscow Russia;</p> <p>A.M. Prokhorov General Physics InstituteRussian Academy of SciencesVavilov str. 38 119991 Moscow Russia;</p> <p>A.M. Prokhorov General Physics InstituteRussian Academy of SciencesVavilov str. 38 119991 Moscow Russia;</p> <p>A.M. Prokhorov General Physics InstituteRussian Academy of SciencesVavilov str. 38 119991 Moscow Russia;</p> <p>A.M. Prokhorov General Physics InstituteRussian Academy of SciencesVavilov str. 38 119991 Moscow Russia;</p> <p>A.M. Prokhorov General Physics InstituteRussian Academy of SciencesVavilov str. 38 119991 Moscow Russia;</p> <p>Joint Institute for Nuclear ResearchJoliot‐Curie str. 6 141980 Dubna Moscow Region Russia;</p> <p>Joint Institute for Nuclear ResearchJoliot‐Curie str. 6 141980 Dubna Moscow Region Russia;</p> <p>Institute for Theoretical and Applied ElectromagneticsRussian Academy of SciencesIzhorskaya str. 13 125412 Moscow Russia;</p> <p>Institute for Theoretical and Applied ElectromagneticsRussian Academy of SciencesIzhorskaya str. 13 125412 Moscow Russia;</p> <p>Institute for Theoretical and Applied ElectromagneticsRussian Academy of SciencesIzhorskaya str. 13 125412 Moscow Russia;</p> <p>Institute for Theoretical and Applied ElectromagneticsRussian Academy of SciencesIzhorskaya str. 13 125412 Moscow Russia;</p> <p>Chemistry DepartmentM.V. Lomonosov Moscow State UniversityLeninskiye Gory 1‐3 119991 Moscow Russia;</p> <p>Chemistry DepartmentM.V. Lomonosov Moscow State UniversityLeninskiye Gory 1‐3 119991 Moscow Russia;</p> <p>N.M. Emanuel Institute of Biochemical PhysicsRussian Academy of SciencesKosygin str. 4 119334 Moscow Russia;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/4724.html" title="光谱学">光谱学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=SECARS&option=203" rel="nofollow">SECARS;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=metamaterial&option=203" rel="nofollow">metamaterial;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Au‐nanoparticles&option=203" rel="nofollow">Au‐nanoparticles;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=CeO 2&option=203" rel="nofollow">CeO 2;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=biosensor&option=203" rel="nofollow">biosensor;</a> </p> <div class="translation"> 机译：Secars;超材料;Au-nanoparticles;CEO 2;生物传感器; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704025815147.html">Surface‐enhanced micro‐ <fc xmlns="http://www.wiley.com/namespaces/wiley">CARS</fc>CARS mapping of a nanostructured cerium dioxide/aluminum film surface with gold nanoparticle‐bound organic molecules</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Fabelinsky Viktor I.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Fabelinsky Viktor I.,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kozlov Dimitrii N.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Kozlov Dimitrii N.,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Orlov Sergey N.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Orlov Sergey N.,</a> <a href="/journal-foreign-35645/" target="_blank" rel="nofollow" class="tuijian_authcolor">Journal of Raman Spectroscopy: An International Journal for Original Work in All Aspects of Raman Spectroscopy, Including Higher Order Processes, and Also Brillouin- and Rayleigh Scattering .</a> <span>2018</span><span>,第7期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：表面增强的微XMLNS =“http://www.wiley.com/namespace/wiley”>汽车</ fc>纳米结构二氧化铈/铝膜表面与金纳米粒子结合的有机分子的车辆映射</span> </p> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704025580408.html">Eddy‐induced sea surface temperature gradients in <fc xmlns="http://www.wiley.com/namespaces/wiley">E</fc>E astern <fc xmlns="http://www.wiley.com/namespaces/wiley">B</fc>B oundary <fc xmlns="http://www.wiley.com/namespaces/wiley">C</fc>C urrent <fc xmlns="http://www.wiley.com/namespaces/wiley">S</fc>S ystems</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yuan Yeping&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Yuan Yeping,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Castelao Renato M.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Castelao Renato M. </a> <a href="/journal-foreign-34643/" target="_blank" rel="nofollow" class="tuijian_authcolor">Journal of Geophysical Research, C. 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href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=王丽华&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,王丽华</a> <span> <a href="/journal-cn-4704/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 山东科技大学学报（自然科学版） </a> </span> <span> . 2019</span><span>,第006期</span> </span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/academic-journal-cn_acta-physica-sinica_thesis/0201271608319.html">聚甲基丙烯酸甲酯间隔的金纳米立方体与金膜复合结构的表面增强拉曼散射研究</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=王向贤&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 王向贤</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=白雪琳&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,白雪琳</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=庞志远&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,庞志远</a> <span> <a href="/journal-cn-15096/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 物理学报 </a> </span> <span> . 2019</span><span>,第003期</span> </span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/academic-journal-cn_journal-xinyang-normal-university-natural-science-edition_thesis/0201295944052.html">自组装二维银纳米粒子的复合Langumir-Blodgett膜的结构及表面增强拉曼散射研究</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=张振龙&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 张振龙</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=万敏&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,万敏</a> <span> <a href="/journal-cn-51016/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 信阳师范学院学报：自然科学版 </a> </span> <span> . 2003</span><span>,第3期</span> </span> </div> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/academic-conference-cn_meeting-11952_thesis/02022512400.html">应用环糊精与金纳米粒子的结合体系对多环芳烃的表面增强拉曼检测</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=谢云飞&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 谢云飞</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=王旭&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,王旭</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=赵冰&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,赵冰</a> <span> <a href="/conference-cn-11952/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 第十六届全国分子光谱学学术会议 </a> <span> <span> . 2010</span> </span> </div> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020312763342.html">金纳米粒子标记结合表面增强拉曼法对蛋白质的检测</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=李桃&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 李桃</a> <span> . 2008</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/061202388654.html">一种用于表面增强拉曼散射的铝纳米结构的制备方法</a> <b>[P]</b> . <span> 中国专利： CN105562936B </span> <span> . 2017.03.29</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120108043797.html">一种用于表面增强拉曼散射的铝纳米结构的制备方法</a> <b>[P]</b> . <span> 中国专利： CN105562936A </span> <span> . 2016-05-11</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130408609071.html">SERS - Plasmonic metal-polymer film hybrid nanostructure which can reversibly modulate Surface Enhanced Raman Scattering SERS signals of organic molecules according to external temperature</a> <b>[P]</b> . <span> 外国专利：  KR101726033B1 </span> <span> . 2017-04-26</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：SERS-等离子金属-聚合物薄膜混合纳米结构，可根据外部温度可逆地调节有机分子的表面增强拉曼散射SERS信号 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130411469774.html">PLASMONIC METAL-POLYMER FILM HYBRID NANOSTRUCTURE WHICH CAN REVERSIBLY MODULATE SURFACE ENHANCED RAMAN SCATTERING (SERS) SIGNALS OF ORGANIC MOLECULES ACCORDING TO EXTERNAL TEMPERATURE</a> <b>[P]</b> . <span> 外国专利：  KR20160087260A </span> <span> . 2016-07-21</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：等离子金属-聚合物薄膜混合纳米结构，可根据外部温度反向调节表面增强的拉曼散射（SERS）信号 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130499629853.html">CALCIUM OXIDE NANOPARTICLES AND POLYMERIC NANOCOMPOSITE COMPRISING SAME, METHOD FOR PRODUCING SAME FROM NATURAL SOLID FOOD BYPRODUCTS/WASTE RICH IN CALCIUM CARBONATE AND METHOD FOR PREPARING THE POLYMERIC NANOCOMPOSITE, AND USE THEREOF AS AN ANTIMICROBIAL AGENT IN FILMS FOR PACKAGING FOOD OR COATINGS FOR VARIOUS SURFACES</a> <b>[P]</b> . <span> 外国专利：  WO2021046661A1 </span> <span> . 2021-03-18</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：包含该氧化钙纳米颗粒和聚合物纳米复合材料，其与富含碳酸钙的天然固体食品副产物/废物的制备方法及其制备聚合物纳米复合材料的方法，以及在薄膜中用作用于包装食品或涂层的抗微生物剂 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704025815147','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: 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Surface‐enhanced micro‐ CARSCARS mapping of a nanostructured cerium dioxide/aluminum film surface with gold nanoparticle‐bound organic molecules

摘要