Statistical analysis of cuboctahedral silver nanocrystals Langmuir–Blodgett film        <fc xmlns='http://www.wiley.com/namespaces/wiley'>SERS</fc>SERS        substrate

Chen Wei‐Liang; Huang Yi‐Hsin; Cheng Hui‐Yu; Kuo Tsung‐Rong; Chang Yu‐Ming

摘要

Abstract >With single‐molecule sensitivity, surface‐enhanced Raman scattering (SERS) has promised to be a powerful tool from chemical analysis to biosensors. However, problem with large signal fluctuations for reproducibility has impeded SERS from widespread application. The fabrication of SERS substrate with large and uniform enhancement in combination with an effective target analyte‐transfer process is crucial for applications of SERS for trace molecule detection. In this study, we performed laser‐scanning confocal mapping to characterize 3 SERS substrate samples. The substrate consists of a monolayer of cuboctahedral silver nanocrystals (AgNCs) made with Langmuir–Blodgett technique. The synthesis of the cuboctahedral AgNCs involves the use of polyvinylpyrrolidone (PVP) as a shape‐controlling agent that remains on the surface of the nanocrystals. Using PVP as an analyte, we investigate the temporal and spatial variation of PVP SERS signals from the cuboctahedral AgNC Langmuir–Blodgett film. Analyzing the enhancement probability distribution with a model allows quantitative characterization of the cuboctahedral AgNC SERS substrates. The results help to identify important SERS substrate characteristics that influence the performance of the SERS substrate. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><abstract xmlns =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <title type =“main”>抽象</ title> >与单个 - 极小的灵敏度，表面增强的拉曼散射（SERS）已承诺是从化学分析到生物传感器的强大工具。然而，具有大量信号波动的问题，用于再现性的潜冲从广泛的应用中阻碍了SERS。与有效目标分析物转移过程的组合具有大和均匀增强的SERS基板对SERS用于痕量分子检测的应用至关重要。在这项研究中，我们执行了激光扫描共焦映射，以表征3个SERS基板样本。基材由用Langmuir-Blodgett技术制成的甲型甲状腺二氢烷纳米晶体（AgNC）的单层组成。 CuboctaheDral AgNC的合成涉及使用聚乙烯吡咯烷酮（PVP）作为形状控制剂，其保留在纳米晶体的表面上。使用PVP作为分析物，研究PVP SERS信号来自CuboctaheDral Agnc Langmuir-Blodgett薄膜的时间和空间变化。分析具有模型的增强概率分布允许群式对二角形AGNC SERS基材的定量表征。结果有助于确定影响SERS基板性能的重要SERS基板特性。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-35645/'>《Journal of Raman Spectroscopy: An International Journal for Original Work in All Aspects of Raman Spectroscopy, Including Higher Order Processes, and Also Brillouin- and Rayleigh Scattering》</a> <b style="margin: 0 2px;">|</b><span>2018年第5期</span><b style="margin: 0 2px;">|</b><span>共8页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Wei‐Liang&option=202" target="_blank" rel="nofollow">Chen Wei‐Liang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huang Yi‐Hsin&option=202" target="_blank" rel="nofollow">Huang Yi‐Hsin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cheng Hui‐Yu&option=202" target="_blank" rel="nofollow">Cheng Hui‐Yu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kuo Tsung‐Rong&option=202" target="_blank" rel="nofollow">Kuo Tsung‐Rong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chang Yu‐Ming&option=202" target="_blank" rel="nofollow">Chang Yu‐Ming;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Center for Condensed Matter SciencesNational Taiwan UniversityTaipei 10617 Taiwan;</p> <p>Center for Condensed Matter SciencesNational Taiwan UniversityTaipei 10617 Taiwan;</p> <p>Center for Condensed Matter SciencesNational Taiwan UniversityTaipei 10617 Taiwan;</p> <p>Graduate Institute of Nanomedicine and Medical Engineering College of Biomedical EngineeringTaipei Medical UniversityTaipei 11031 Taiwan;</p> <p>Center for Condensed Matter SciencesNational Taiwan UniversityTaipei 10617 Taiwan;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/4724.html" title="光谱学">光谱学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=enhancement probability distribution&option=203" rel="nofollow">enhancement probability distribution;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=laser‐scanning confocal spectromicroscope&option=203" rel="nofollow">laser‐scanning confocal spectromicroscope;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=polyvinylpyrrolidone&option=203" rel="nofollow">polyvinylpyrrolidone;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=signal fluctuation&option=203" rel="nofollow">signal fluctuation;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=surface‐enhanced Raman scattering ( SERS )&option=203" rel="nofollow">surface‐enhanced Raman scattering ( SERS );</a> </p> <div class="translation"> 机译：增强概率分布;激光扫描共聚焦光谱显微镜;聚乙烯吡咯烷酮;信号波动;表面增强拉曼散射（SERS）; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li 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Statistical analysis of cuboctahedral silver nanocrystals Langmuir–Blodgett film SERSSERS substrate

摘要