Heterogeneous and homogeneous photocatalytic degradation of psychoactive drug Fluvoxamine: kinetic study, inorganic ions and phytotoxicity evaluation

Tsoumachidou Sophia; Kouras Athanasios; Poulios Ioannis

摘要

Abstract <section xml:id="jctb5543-sec-0001" numbered="no"> <title type="main" xml:lang="de">BACKGROUND >Pharmaceutically active compounds, emerging extensively in ecosystems as pollutants, have become an important environmental and public health issue, since they can contaminate drinking water and pose threats to wildlife and human health. As a result, efforts should be made to develop methods to inactivate or eliminate this class of substance in the environment. </section> <section xml:id="jctb5543-sec-0002" numbered="no"> <title type="main">RESULTS > The photocatalytic degradation of psychoactive drug Fluvoxamine has been investigated. In the case of heterogeneous photocatalytic oxidation, the effect of TiO <sub>2</sub> P25 concentration (0.1–1?g L ‐1 ), initial concentration of H <sub>2</sub> O <sub>2</sub> (0.25–0.2?g L ‐1 ) and Fe 3+ (0.00175–0.014?g L ‐1 ) and pH of the solution on initial reaction rates were evaluated, while for homogeneous photocatalytic oxidation the effect of the amount of H <sub>2</sub> O <sub>2</sub> (0.25–0.2?g L ‐1 ) and Fe 3+ (0.00175–0.014?g L ‐1 ) were investigated. In addition, the conversion of the heteroatoms in the FVX molecule to inorganic ions (NO <sub>3</sub> ‐ , NH <sub>4</sub> + , F ‐ ) during the photocatalytic process has been observed and phytotoxici </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <title type =“main”>抽象</ title> <section XML：ID =“JCTB5543-SEC-0001”编号=“否”> <标题类型=“Main”XML：Lang =“de”>背景</标题> >药物活性化合物，广泛地在生态系统中作为污染物出现，已成为重要的环境和公共卫生问题，因为他们可以污染饮用水并对野生动物和人类健康构成威胁。因此，应努力制定在环境中灭活或消除这类物质的努力。</ p> </段> <部分XML：ID =“JCTB5543-SEC-0002”编号=“否”> <标题类型=“main”>结果</标题> >已经研究了精神毒性药物氟胺的光催化降解。在非均相光催化氧化的情况下，TiO <sub> 2 </ sub> p25浓度的影响（0.1-1〜g l -1 </ sup>），H <sub> 2的初始浓度</ Sub> O <sub> 2 </ sub>（0.25-0.2〜g l -1-sup>）和Fe 3 + </ sup>（0.00175-0.014≤gl - 评价初始反应速率的溶液的1 </ sup>）和pH值，而均匀的光催化氧化H <sub> 2 </ sub> O <sub> 2 </ sub>的效果（0.25-研究了0.2〜G L <SUP> -1℃和Fe 3 + </ sup>（0.00175-0.014？g l -1 </ sup>）。另外，将FVX分子中的杂原子转化为无机离子（NO <sub> 3 </ sub> - ，NH <sub> 4 </ sub> + </ sup观察到光催化过程中的F - </ sup>）和phytotoxici </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-33908/'>《Journal of Chemical Technology & Biotechnology》</a> <b style="margin: 0 2px;">|</b><span>2018年第6期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tsoumachidou Sophia&option=202" target="_blank" rel="nofollow">Tsoumachidou Sophia;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kouras Athanasios&option=202" target="_blank" rel="nofollow">Kouras Athanasios;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Poulios Ioannis&option=202" target="_blank" rel="nofollow">Poulios Ioannis;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Laboratory of Physical Chemistry Department of ChemistryAristotle University of ThessalonikiThessaloniki Greece;</p> <p>Laboratory of Physical Chemistry Department of ChemistryAristotle University of ThessalonikiThessaloniki Greece;</p> <p>Laboratory of Physical Chemistry Department of ChemistryAristotle University of ThessalonikiThessaloniki Greece;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/180.html" title="生物工程学（生物技术）">生物工程学（生物技术）;</a><a href="https://www.zhangqiaokeyan.com/clc/20827.html" title="生物化学过程">生物化学过程;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=fluvoxamine&option=203" rel="nofollow">fluvoxamine;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=psychoactive drug&option=203" rel="nofollow">psychoactive drug;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=urban wastewater&option=203" rel="nofollow">urban wastewater;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=photocatalytic oxidation&option=203" rel="nofollow">photocatalytic oxidation;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=TiO 2&option=203" rel="nofollow">TiO 2;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=photo‐Fenton&option=203" rel="nofollow">photo‐Fenton;</a> </p> <div class="translation"> 机译：Fluvoxamine;精神毒品;城市废水;光催化氧化;TiO 2;照片芬顿; 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