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C/ZTS e solar cells developed on polymer substrates: Effects of low‐temperature processing

机译：C / ZTS E在聚合物基材上开发的太阳能电池：低温加工的影响

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Abstract > Cu <sub>2</sub> ZnSn(S <sub>1?x</sub> Se <sub>x</sub> ) <sub>4</sub> solar cells are well suited for roll‐to‐roll mass production since they are formed mainly by non‐toxic and earth‐abundant elements. Polyimide (PI) has proved to be a promising roll‐to‐roll compatible substrate yielding very high efficiency devices for Cu(In,Ga)Se <sub>2</sub> . In this work, we demonstrate the feasibility of using PI as a low‐weight and flexible alternative to soda‐lime glass for Cu <sub>2</sub> ZnSnSe <sub>4</sub> (CZTSe) solar cells. Two main concerns arise when working with PI. Firstly, its low thermal robustness limits process temperatures below 500°C. The second concern is the lack of alkali in PI in contrast to conventional soda‐lime glass fundamental for high efficiency devices. This work tackles both issues. First, different alkali doping strategies are investigated for the incorporation of Na and K into CZTSe absorbers prepared on PI substrates by sequential precursor sputtering and selenization at 470°C: pre‐absorber synthesis and post‐deposition treatment. Post‐deposition treatment does not lead to an improvement of performance. Pre‐absorber synthesis effectively dopes the CZTSe absorbers increasing the solar cell performance and carrier concentration of the devices. Cu <sub>2</sub> ZnSnSe <sub>4</sub> devices are then fabricated on glass and PI at different temperatures (450°C‐490°C). A detrimental SnSe <sub>2</sub> secondary phase is detected in most of these devices. The formation of this phase is proved to be strongly related to process temperature. Despite this, a 6.4% efficiency device is achieved at 490°C on glass. Finally, through further experimentation and the addition of a Ge nanolayer, we report a 4.9% efficiency flexible device on PI setting a new record for kesterite solar cells on a polymer substrate. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > CU. <sub> 2 </ sub> znsn（S. <sub> 1？x </ sub> se <sub> x </ sub> 的） <sub> 4 </ sub> 太阳能电池非常适合于卷料批量生产，因为它们主要由无毒和土坯元素形成。已证明聚酰亚胺（PI）是一种有前途的卷载兼容底物，其产生非常高效的Cu（In，Ga）Se <sub> 2 </ sub> 。在这项工作中，我们证明了使用PI作为苏打水玻璃的低重量和柔性替代品的可行性 <sub> 2 </ sub> znsnse. <sub> 4 </ sub> （CZTSE）太阳能电池。使用PI时出现两个主要问题。首先，其低热稳健性限制了500℃以下的过程温度。第二个问题是与常规钠钙玻璃对高效装置的缺乏碱性碱性碱性。这项工作解决了两个问题。首先，研究了不同的碱掺杂策略以通过在470℃下序列化的前体溅射和硒化在470℃下硒化和沉积后处理和沉积后处理，将Na和k掺入CZTSE吸收剂。沉积后治疗不会导致性能的提高。预吸收剂合成有效地掺杂CZTSE吸收剂，增加了装置的太阳能电池性能和载体浓度。 CU. <sub> 2 </ sub> znsnse. <sub> 4 </ sub> 然后在不同温度（450℃-490℃）的玻璃和PI上制造装置。一个有害的桑斯 <sub> 2 </ sub> 在大多数这些设备中检测二次相位。证明该阶段的形成是与过程温度强烈相关的。尽管如此，在490°C上实现了6.4％的效率装置。最后，通过进一步的实验和加入GE纳米层，我们在PI上报告了4.9％的效率灵活装置，在聚合物基板上设置了KETERITE太阳能电池的新记录。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-29870/'>《Progress in photovoltaics》</a> <b style="margin: 0 2px;">|</b><span>2018年第1期</span><b style="margin: 0 2px;">|</b><span>共14页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Becerril‐Romero Ignacio&option=202" target="_blank" rel="nofollow">Becerril‐Romero Ignacio;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Acebo Laura&option=202" target="_blank" rel="nofollow">Acebo Laura;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Oliva Florian&option=202" target="_blank" rel="nofollow">Oliva Florian;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Izquierdo‐Roca Víctor&option=202" target="_blank" rel="nofollow">Izquierdo‐Roca Víctor;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=López‐Marino Simón&option=202" target="_blank" rel="nofollow">López‐Marino Simón;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Espíndola‐Rodríguez Moisés&option=202" target="_blank" rel="nofollow">Espíndola‐Rodríguez Moisés;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Neuschitzer Markus&option=202" target="_blank" rel="nofollow">Neuschitzer Markus;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sánchez Yudania&option=202" target="_blank" rel="nofollow">Sánchez Yudania;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Placidi Marcel&option=202" target="_blank" rel="nofollow">Placidi Marcel;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Pérez‐Rodríguez Alejandro&option=202" target="_blank" rel="nofollow">Pérez‐Rodríguez Alejandro;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Saucedo Edgardo&option=202" target="_blank" rel="nofollow">Saucedo Edgardo;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Pistor Paul&option=202" target="_blank" rel="nofollow">Pistor Paul;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>IREC ‐ Catalonia Institute for Energy ResearchSant Adrià de Besòs Spain;</p> <p>IREC ‐ Catalonia Institute for Energy ResearchSant Adrià de Besòs Spain;</p> <p>IREC ‐ Catalonia Institute for Energy ResearchSant Adrià de Besòs Spain;</p> <p>IREC ‐ Catalonia Institute for Energy ResearchSant Adrià de Besòs Spain;</p> <p>IREC ‐ Catalonia Institute for Energy ResearchSant Adrià de Besòs Spain;</p> <p>IREC ‐ Catalonia Institute for Energy ResearchSant Adrià de Besòs Spain;</p> <p>IREC ‐ Catalonia Institute for Energy ResearchSant Adrià de Besòs Spain;</p> <p>IREC ‐ Catalonia Institute for Energy ResearchSant Adrià de Besòs Spain;</p> <p>IREC ‐ Catalonia Institute for Energy ResearchSant Adrià de Besòs Spain;</p> <p>IREC ‐ Catalonia Institute for Energy ResearchSant Adrià de Besòs Spain;</p> <p>IREC ‐ Catalonia Institute for Energy ResearchSant Adrià de Besòs Spain;</p> <p>IREC ‐ Catalonia Institute for Energy ResearchSant Adrià de Besòs Spain;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/7667.html" title="通信系统（传输系统）">通信系统（传输系统）;</a><a href="https://www.zhangqiaokeyan.com/clc/1790.html" title="光电子技术、激光技术">光电子技术、激光技术;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=alkali doping&option=203" rel="nofollow">alkali doping;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=CZTS e&option=203" rel="nofollow">CZTS e;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=kesterite solar cells&option=203" rel="nofollow">kesterite solar cells;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=low temperature&option=203" rel="nofollow">low temperature;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=polyimide substrate&option=203" rel="nofollow">polyimide substrate;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=S n S e 2 secondary phase&option=203" rel="nofollow">S n S e 2 secondary phase;</a> </p> <div class="translation"> 机译：碱掺杂;CZTS E;kesterite太阳能电池;低温;聚酰亚胺衬底;S N S E 2二次相; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" 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href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=袁春伟&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,袁春伟</a> <span> <a href="/conference-cn-27227/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 2004年中国材料研讨会 </a> <span> <span> . 2004</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020312147954.html">溶液加工的阴极修饰层对聚合物太阳能电池性能的影响</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=姜亮&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 姜亮</a> <span> . 2012</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/061201879257.html">位于具有可由溶液低温加工的电介质的机械柔性聚合物衬底上的金属氧化物场效应晶体管</a> <b>[P]</b> . <span> 中国专利： CN102668086B </span> <span> . 2016.01.06</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120106849949.html">位于具有可由溶液低温加工的电介质的机械柔性聚合物衬底上的金属氧化物场效应晶体管</a> <b>[P]</b> . <span> 中国专利： CN102668086A </span> <span> . 2012-09-12</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130435940696.html">LOW-REFLECTANCE PROCESSING METHOD OF SILICON SUBSTRATE FOR SOLAR CELLS AND SILICON SUBSTRATE FOR SOLAR CELL</a> <b>[P]</b> . <span> 外国专利：  JP2007036170A </span> <span> . 2007-02-08</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：太阳电池硅基质的低反射率处理方法和太阳能电池硅基质的低反射率处理方法 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130424532006.html">METHOD FOR DEVELOPING A RESIST FILM ON A SUBSTRATE USING A DEVELOPER WITH LOWER TEMPERATURE THAN ROOM TEMPERATURE, A COMPUTER STORAGE APPARATUS, AND A DEVELOPING PROCESS SYSTEM</a> <b>[P]</b> . <span> 外国专利：  KR20110087201A </span> <span> . 2011-08-02</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：使用比室温低的温度的显影剂在基材上显影抗蚀膜的方法，计算机存储装置以及显影过程系统 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130400869491.html">CONJUGATED POLYMER FOR LOW-TEMPERATURE PROCESSING, AND ORGANIC SOLAR CELL USING SAME</a> <b>[P]</b> . <span> 外国专利：  WO2020171320A1 </span> <span> . 2020-08-27</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：用于低温加工的共轭聚合物，以及使用相同的有机太阳能电池 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon 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