Rheo‐Raman spectroscopic study of microscopic deformation behavior for ultra‐low‐density polyethylene

Kida Takumitsu; Hiejima Yusuke; Nitta Koh‐hei

摘要

Abstract > <fi>In situ</fi> Raman spectroscopy was applied to ultra‐low‐density polyethylene (ULDPE) to investigate the microscopic deformation behavior under uniaxial stretching. It was found that the crystalline chains of ULDPE show a bimodal molecular orientation parallel and perpendicular to the stretching direction beyond the elastic region. The peak shifts of C???C stretching modes of the crystalline chains obviously depend on the polarization direction, suggesting that the microscopic load sharing is anisotropic. Whereas the stretching stress is applied on the crystalline chains oriented in the stretching direction, the compression stress is applied on those oriented perpendicular to the stretching direction. This anisotropic load sharing is caused by the Poisson shrinkage of the specimen owing to the rubber‐like properties of ULDPE. ? 2018 Society of Chemical Industry </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <标题类型=“main”>抽象</ title> > <fi>原位</ fi> 将拉曼光谱应用于超低密度聚乙烯（ULDPE），以研究单轴拉伸下的微观变形行为。发现ULDPE的结晶链显示了平行的双峰分子取向，垂直于弹性区域之外的拉伸方向。 C ??? C的峰值偏移模式的结晶链显然取决于偏振方向，表明微观载荷共享是各向异性的。虽然施加在拉伸方向上取向的晶体链上的拉伸应力，则压缩应力施加在垂直于拉伸方向上的那些。这种各向异性负载分配是由于ULDPE的橡胶状性能所造的泊松收缩。还2018年化学工业学会 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-29710/'>《Polymer international》</a> <b style="margin: 0 2px;">|</b><span>2018年第10期</span><b style="margin: 0 2px;">|</b><span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kida Takumitsu&option=202" target="_blank" rel="nofollow">Kida Takumitsu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hiejima Yusuke&option=202" target="_blank" rel="nofollow">Hiejima Yusuke;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Nitta Koh‐hei&option=202" target="_blank" rel="nofollow">Nitta Koh‐hei;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Chemical and Materials ScienceKanazawa University KakumaKanazawa Japan;</p> <p>Department of Chemical and Materials ScienceKanazawa University KakumaKanazawa Japan;</p> <p>Department of Chemical and Materials ScienceKanazawa University KakumaKanazawa Japan;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1185.html" title="高分子化学（高聚物）">高分子化学（高聚物）;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Raman spectroscopy&option=203" rel="nofollow">Raman spectroscopy;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=rheo‐optics&option=203" rel="nofollow">rheo‐optics;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=deformation behavior&option=203" rel="nofollow">deformation behavior;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=ULDPE&option=203" rel="nofollow">ULDPE;</a> </p> <div class="translation"> 机译：拉曼光谱;Rheo-Optics;变形行为;ULDPE; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> 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