Measurement of photo-neutron cross sections and isomeric yield ratios in the 89Y(γ,xn)89?x Y reactions at the bremsstrahlung end-point energies of 65, 70 and 75 MeV

摘要

The flux-weighted average cross sections of the 89Y(γ,xn; x=1–4)89?x Y reactions and the isomeric yield ratios of the 87m,gY, 86m,gY, and 85m,gY radionuclides produced in these reactions with the bremsstrahlung end-point energies of 65, 70 and 75 MeV have been determined by an activation and off-line γ-ray spectrometric technique using the 100 MeV electron linac in Pohang Accelerator Laboratory, Korea. The theoretical 89Y(γ,xn; x=1–4)89?x Y reactioncross sections for mono-energetic photonshave been calculated using the computer code TALYS 1.6. Then the flux-weighted theoretical values were obtaind to compare with the present data. The flux-weighted experimental and theoretical 89Y(γ,xn; x=1–4)89?x Y reaction cross sections increase very fast from the threshold values to a certain bremsstrahlung energy, wherethe other reaction channels open up. Thereafter it remains constant a while and then slowly decreases with the increase of cross sections for other reactions. Similarly, the isomeric yield ratios of 87m,gY,86m,gY and 85m,gY in the 89Y(γ,xn; x=2–4)89?x Y reactions from the present work and literature data show an increasing trend from their respective threshold values to a certain bremsstrahlung energy. After a certain point ofenergy, the isomeric yield ratios increase slowly with the bremsstrahlung energy. These observations indicate the role of excitation energy and its partitioning in different reaction channels.