Ordering pH‐Responsive Polyelectrolyte‐Grafted Nanoparticles in a Flow Coating Process

Zhang Chongfeng; Carlson Thomas; Yang Siyang; Akcora Pinar

摘要

Abstract >The effects of nanoscale particle interactions on deposition patterns in the flow coating process are investigated using pH‐responsive poly(acrylic acid) (PAA)‐grafted silica nanoparticles. Interactions between nanoparticles are effectively controlled by grafting densities, PAA brush lengths, and pH, in addition to hydrogen bonding between free polyvinylpyrrolidone (PVP) and PAA. Consequently, various intriguing patterns of randomly distributed dots, polygonal networks, meshes, fork‐like structures along with highly regulated and densely packed stripes parallel to the moving direction of substrates are fabricated. Per se, the flow coating process is shown to form regulated patterns during evaporation by controlling particle–particle interactions with inherent brush properties and external pH. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> >使用pH-响应聚（丙烯酸）（PAA） - 移植的二氧化硅纳米粒子研究了纳米级颗粒相互作用对流动涂覆工艺中的沉积图案的影响。除了自由聚乙烯吡咯烷酮（PVP）和PAA之间的氢键合之外，纳米颗粒之间的相互作用是通过接枝密度，PAA刷长和pH有效控制。因此，制造了随机分布点，多边形网络，网格，叉状结构以及与基板的移动方向平行的高度调节和密集的填充条纹的各种诱人的诱人图案。本身，通过控制与固有刷性能和外部pH的颗粒颗粒相互作用控制蒸发过程中的流动涂布过程以形成调节图案。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2018年第5期</span><b style="margin: 0 2px;">|</b><span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Chongfeng&option=202" target="_blank" rel="nofollow">Zhang Chongfeng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Carlson Thomas&option=202" target="_blank" rel="nofollow">Carlson Thomas;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Siyang&option=202" target="_blank" rel="nofollow">Yang Siyang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Akcora Pinar&option=202" target="_blank" rel="nofollow">Akcora Pinar;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Chemical Engineering and Materials ScienceStevens Institute of TechnologyHoboken NJ 07030 USA;</p> <p>Department of Chemical Engineering and Materials ScienceStevens Institute of TechnologyHoboken NJ 07030 USA;</p> <p>Department of Chemical Engineering and Materials ScienceStevens Institute of TechnologyHoboken NJ 07030 USA;</p> <p>Department of Chemical Engineering and Materials ScienceStevens Institute of TechnologyHoboken NJ 07030 USA;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=flow coating&option=203" rel="nofollow">flow coating;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=grafted nanoparticles&option=203" rel="nofollow">grafted nanoparticles;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=particle–particle interactions&option=203" rel="nofollow">particle–particle interactions;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=pH‐responsive polyelectrolyte&option=203" rel="nofollow">pH‐responsive polyelectrolyte;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=self‐assembly&option=203" rel="nofollow">self‐assembly;</a> </p> <div class="translation"> 机译：流动涂层;接枝纳米颗粒;颗粒颗粒相互作用;pH响应聚电解质;自组装; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 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CHEN Ye</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=陈叶&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,陈叶</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=FANG Wenxiang&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,FANG Wenxiang</a> <span> <a href="/conference-cn-8551/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 2012年全国高分子材料科学与工程研讨会 </a> <span> <span> . 2012</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020314946354.html">RAFT可控聚合聚电解质及其与无机多孔材料复合构建pH响应离子传输通道研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=戴道兴&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 戴道兴</a> <span> . 2013</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120879754.html">pH响应型两亲接枝聚膦腈给药胶束及其制备方法</a> <b>[P]</b> . <span> 中国专利： CN101785865B </span> <span> . 2012.02.15</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120848769.html">pH响应型两亲接枝聚膦腈及其合成方法</a> <b>[P]</b> . <span> 中国专利： CN101759855B </span> <span> . 2011.12.14</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130441410076.html">Heat exchanger for vehicle comprises a hydrophilic surface coating containing nanoparticles, coated nanoparticles and/or grafted nanoparticles with or made from oxides</a> <b>[P]</b> . <span> 外国专利：  DE102004011545A1 </span> <span> . 2004-10-14</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：用于车辆的热交换器包括亲水性表面涂层，该亲水性表面涂层包含纳米颗粒，涂覆的纳米颗粒和/或具有或由氧化物制成的接枝的纳米颗粒 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130417284673.html">VISIBLE-LIGHT-RESPONSIVE PHOTOCATALYST POWDER, PROCESS FOR PRODUCING THE SAME, AND VISIBLE-LIGHT-RESPONSIVE PHOTOCATALYST MATERIAL, PHOTOCATALYTIC COATING MATERIAL, AND PHOTOCATALYTIC PRODUCT EACH CONTAINING THE SAME</a> <b>[P]</b> . <span> 外国专利：  EP2186560A4 </span> <span> . 2013-12-25</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：可见光响应性光催化剂粉末，其制备方法以及可见光响应性光催化剂材料，光催化涂层材料和包含该光催化剂的光催化产品 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130427185044.html">VISIBLE-LIGHT-RESPONSIVE PHOTOCATALYST POWDER, PROCESS FOR PRODUCING THE SAME, AND VISIBLE-LIGHT-RESPONSIVE PHOTOCATALYST MATERIAL, PHOTOCATALYTIC COATING MATERIAL, AND PHOTOCATALYTIC PRODUCT EACH CONTAINING THE SAME</a> <b>[P]</b> . <span> 外国专利：  EP2186560A1 </span> <span> . 2010-05-19</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：可见光响应性光催化剂粉末，其制备方法以及可见光响应性光催化剂材料，光催化涂层材料和包含该光催化剂的光催化产品 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704022435548','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img src="https://cdn.zhangqiaokeyan.com/img/loginclose.png" alt="关闭" onclick="$('.journalsub-pop-up').hide()"> <p 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