Amino Acid Immobilization of Copper Surface Diffusion on Cu(111)

Guisinger Nathan P.; Mannix Andrew J.; Rankin Rees B.; Kiraly Brian; Phillips Jesse A.; Darling Seth B.; Fisher Brandon L.; Hersam Mark C.; Iski Erin V.

摘要

Abstract >Surface diffusion and molecular self‐assembly are two critically important processes in chemistry and nature. Amino acids deposited on a Cu(111) surface driving a separation at the 2D limit between self‐assembling molecules and diffusing copper atoms is reported. Since the self‐assembling amino acids prefer non‐planar, tridentate bonding with neighboring adatoms, they attach to and immobilize diffusing copper adatoms on the surface. This chemical interaction freezes out the copper diffusion causing the condensation of “solid” copper adatom islands on the surface. Such separation and immobilization are observed for eight different amino acids, suggesting the generality of this phenomenon beyond a single amino acid species. Furthermore, at elevated temperatures, a disruption of the prototypical Ostwald ripening of adatom islands is also observed. These results provide fundamental insight into chiral molecular self‐assembly and its interplay with metal atom surface diffusion. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> 表面扩散和分子自组装是化学和性质中的两个关键重要的方法。据报道，沉积在Cu（111）表面上的氨基酸驱动在自组装分子和扩散铜原子之间的2D极限处的分离。由于自组装氨基酸更喜欢与相邻的adatoms的非平面，因此将其连接并固定在表面上的扩散铜adatoms。这种化学相互作用冻结了铜扩散，导致表面上的“固体”铜Adatom岛的冷凝。对于八种不同的氨基酸观察到这种分离和固定，表明这种现象的一般性超出了单个氨基酸物种。此外，在高温下，还观察到在升高的温度下，也观察到ADATOM岛的原型骨瓦德的破坏。这些结果为手性分子自组装和金属原子表面扩散的相互作用提供了基本的洞察力。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2019年第7期</span><b style="margin: 0 2px;">|</b><span>共8页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Guisinger Nathan P.&option=202" target="_blank" rel="nofollow">Guisinger Nathan P.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Mannix Andrew J.&option=202" target="_blank" rel="nofollow">Mannix Andrew J.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Rankin Rees B.&option=202" target="_blank" rel="nofollow">Rankin Rees B.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kiraly Brian&option=202" target="_blank" rel="nofollow">Kiraly Brian;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Phillips Jesse A.&option=202" target="_blank" rel="nofollow">Phillips Jesse A.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Darling Seth B.&option=202" target="_blank" rel="nofollow">Darling Seth B.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Fisher Brandon L.&option=202" target="_blank" rel="nofollow">Fisher Brandon L.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hersam Mark C.&option=202" target="_blank" rel="nofollow">Hersam Mark C.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Iski Erin V.&option=202" target="_blank" rel="nofollow">Iski Erin V.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Center for Nanoscale MaterialsArgonne National Laboratory9700 South Cass Avenue Building 440 Argonne IL 60439 USA;</p> <p>Center for Nanoscale MaterialsArgonne National Laboratory9700 South Cass Avenue Building 440 Argonne IL 60439 USA;</p> <p>Department of Chemical EngineeringVillanova University800 E Lancaster Ave Villanova PA 19085 USA;</p> <p>Center for Nanoscale MaterialsArgonne National Laboratory9700 South Cass Avenue Building 440 Argonne IL 60439 USA;</p> <p>Department of Chemistry and BiochemistryThe University of Tulsa800 South Tucker Drive Tulsa OK 74104 USA;</p> <p>Chemical Sciences &</p> <p>Engineering DivisionArgonne National Laboratory9700 South Cass Avenue Lemont IL 60439 USA;</p> <p>Center for Nanoscale MaterialsArgonne National Laboratory9700 South Cass Avenue Building 440 Argonne IL 60439 USA;</p> <p>Department of Materials Science and EngineeringNorthwestern University2220 Campus Drive Evanston IL 60208 USA;</p> <p>Department of Chemistry and BiochemistryThe University of Tulsa800 South Tucker Drive Tulsa OK 74104 USA;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=adatoms&option=203" rel="nofollow">adatoms;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=amino acids&option=203" rel="nofollow">amino acids;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cu(111)&option=203" rel="nofollow">Cu(111);</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=LT UHV‐STM&option=203" rel="nofollow">LT UHV‐STM;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=metal surface diffusion&option=203" rel="nofollow">metal surface diffusion;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=metal transport&option=203" rel="nofollow">metal transport;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=molecular assembly&option=203" rel="nofollow">molecular assembly;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=self‐assembly&option=203" rel="nofollow">self‐assembly;</a> </p> <div class="translation"> 机译：吸附剂;氨基酸;Cu（111）;LT UHV-STM;金属表面扩散;金属运输;分子组装;自组装; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022434939.html">Immobilized Cu 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href="/academic-journal-cn_journal-shihezi-university-natural-science_thesis/0201248705327.html">氧原子在Al(111)表面扩散的第一性原理研究</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=魏丽静&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 魏丽静</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=代秀红&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,代秀红</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=郭建新&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,郭建新</a> <span> <a href="/journal-cn-4566/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 石河子大学学报（自然科学版） </a> </span> <span> . 2013</span><span>,第002期</span> </span> </div> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/academic-journal-cn_acta-scientiarum-naturalium-universitatis-nankaiensis_thesis/0201250307060.html">Cu(111)、Ni(111)和Pd(111)催化水煤气变换反应活性的反应能学分析</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=王贵昌&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 王贵昌</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=石全珍&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,石全珍</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=杨作银&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,杨作银</a> <span> <a href="/journal-cn-4679/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 南开大学学报（自然科学版） </a> </span> <span> . 2001</span><span>,第001期</span> </span> </div> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/academic-journal-cn_chinese-journal-inorganic-chemistry_thesis/0201250738430.html">由氨基酸配位的铜修饰十二核钨单元构成的一维链状化合物(H3O)3{Na3(H2O)13(Cu(Gly)2)2(H2W12O42)}·11H2O</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=吴小园&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 吴小园</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=张全争&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,张全争</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=何翔&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,何翔</a> <span> <a href="/journal-cn-15070/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 无机化学学报 </a> </span> <span> . 2006</span><span>,第008期</span> </span> </div> </li> <li> <div> <b>6. </b><a class="enjiyixqcontent" href="/academic-conference-cn_meeting-31760_thesis/02022437897.html">金电极上的氢析出反应中吸附氢原子的表面扩散-析出机理及表面扩散系数的测量</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=苏磊&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 苏磊</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=吴秉亮&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,吴秉亮</a> <span> <a href="/conference-cn-31760/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 第十一次全国电化学会议 </a> <span> <span> . 2001</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020314978988.html">Cu（111）表面扩散势垒的DFT研究和长程相互作用的kMC模拟</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=胡娟梅&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 胡娟梅</a> <span> . 2007</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/061204081475.html">一种制备大面积铜Cu（111）单晶的方法</a> <b>[P]</b> . <span> 中国专利： CN110273176B </span> <span> . 2020.11.03</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120101094078.html">一种制备大面积铜Cu（111）单晶的方法</a> <b>[P]</b> . <span> 中国专利： CN110273176A </span> <span> . 2019-09-24</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130417748684.html">Processes for the preparation of D - 1,2,4 - butanotriol trinitrate 1,2,4 - butanotriol, acid (D - 3.4 - diidroxibutanu00d3ico, acid 3 - desoxi - D - gliceropentanu00d3ico, acid (4S) - 2 - amino - 4 - diidroxipentanu00d3ico; D - 1,2,4 - butanotriol trimethylolethane (D - 1,2,4 - butanotriol, D - xylose dehydrogenase, acid. D - xilu00d4nico, desidratase acid, 3 - desoxi - gliceropentanu00d3ico acid, D - 3 - 4 - diidroxibutanu00d3ico,Acid (4S) - 2 - amino - 4 - diidroxipentanu00d3ico; acids nuclu00c9icos encoders of a D - xylose or recombinant for biossu00cdntese of 1,2,4 - butanotriol, caffeic acid (4S) - 2 - amino - 4 - diidroxipentanu00d3ico, acid (D - 3 - 4 - diidroxibutanu00d3ico, caffeic acid (4S) - 2 - amino - 4.5 - diidroxipentanu00d3ico vector knock-out; A 3 - desoxi - D - glicero - pentulossonato aldolase, entity cell recombinant, cu00c9lula recombinant.The process for research of polinucleotu00cddeos candidates encoding enzymes, antibody.</a> <b>[P]</b> . <span> 外国专利：  BRPI0714439A2 </span> <span> . 2014-04-08</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：D-1,2,4-丁酸三硝酸丁酯1,2,4-丁酸的制备方法（D-3.4-diidroxibutan u00d3ico，酸3-脱氧-D-gliceropentan u00d3ico，酸（4S）-2 -氨基-4-diidroxipentan u00d3ico; D-1,2,4-丁三醇三羟甲基乙烷（D-1,2,4-丁三醇，D-木糖脱氢酶，酸.D-xil u d00nico，desidratase酸，3-脱氧- gliceropentan u00d3ico酸，D-3-4-二溴代丁烷 u00d3ico，酸（4S）-2-氨基-4-diidroxipentan u00d3ico; D-木糖或重组体的酸nucl u00c9icos编码器，1,2 ，4-丁三醇，咖啡酸（4S）-2-氨基-4-二溴代西an丹 u00d3ico，酸（D-3-4-diidroxibutan u00d3ico，咖啡酸（4S）-2-氨基-4.5-diidroxipentan u00d3ico -out; A 3-去氧-D -glicero-戊糖醛酸钠醛缩酶，实体细胞重组体，c9重组体。研究编码酶，抗体的多核苷酸候选物的方法。 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130416878539.html">The copper and copper alloy surface treating Cu-flux for excellent anti-oxidation and anti-grease capability and a surface treating method using the Cu-flux</a> <b>[P]</b> . <span> 外国专利：  KR101342483B1 </span> <span> . 2013-12-17</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：具有优异的抗氧化和抗油脂能力的铜和铜合金表面处理铜焊剂以及使用该铜焊剂的表面处理方法 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130440114347.html">Catalyst for ethylene oxocloracion of 1,2-dichloroethane.Where the distribution of Copper is such that the relationship between X and the concentration of the Copper Atoms Surface given by the ratio of al / Cu (X) on the surface and the given by al / cu</a> <b>[P]</b> . <span> 外国专利：  CL2004000699A1 </span> <span> . 2005-01-21</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：1,2-二氯乙烷的乙烯氧杂环丁烷催化剂，其中铜的分布应使得X与铜原子表面浓度之间的关系由表面上的Al / Cu（X）的比给出，并由铝 /铜 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> 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