Viologen‐Hypercrosslinked Ionic Porous Polymer Films as Active Layers for Electronic and Energy Storage Devices

Wang Luxin; Ding Junjie; Sun Sai; Zhang Bin; Tian Xiangyu; Zhu Jinhui; Song Sannian; Liu Bo; Zhuang Xiaodong; Chen Yu

摘要

Abstract > Over the past decades, numerous scientists have focused on designing complicated monomers, developing new synthesis protocols, and optimizing chemical structures for realizing high‐performance organic or polymer electronics and energy storage devices. However, much less attention has been paid to ionic‐ and radical‐rich porous organic films, which are essential components of aforementioned devices. In this study, an air‐stable, large‐area, free‐standing, and viologen‐linked ionic porous polymer (denoted as IPP‐V) film is developed in situ through electrochemical polymerization. This film is applied to a device by sandwiching it between indium tin oxide (ITO) and Au (i.e., ITO/IPP‐V/Au); the device exhibits a memristive behavior with an ON–OFF current ratio of ≈2. After the IPP‐V film is subjected to thermal pyrolysis at 500 °C, the as‐produced film (denoted as IPP‐V‐500) acts as an active material for an in‐plane micro‐supercapacitor and exhibits a high volumetric capacitance level of up to 4.44 F cm ?3 . This work not only offers a new and convenient strategy toward large‐area ionic porous polymer films for memristor, but also provides a new porous polymer derived carbon film for energy storage. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 在过去的几十年中，许多科学家们侧重于设计复杂的单体，开发新的合成方案，以及优化用于实现高性能有机或聚合物电子和能量存储装置的化学结构。然而，对离子和自由基的多孔有机薄膜进行了更少的注意，这是上述器件的必需组分。在该研究中，通过电化学聚合原位开发出空气稳定，大面积，独立和Viololgen连接的离子多孔聚合物（表示为IPP-V）膜。通过将该薄膜夹在氧化铟锡（ITO）和Au（即，ITO / IPP-V / AU）之间施加到装置上;该器件表现出具有≈2的开关电流比的铭文行为。在500℃的IPP-V膜进行热热解之后，制备的薄膜（表示为IPP-V-500）用作面内微型超级电容器的活性材料，并且表现出高容量电容水平高达4.44 f cm ？3 </ sup> 。这项工作不仅为椎间盘的大面积离子多孔聚合物薄膜提供了一种新的和方便的策略，而且还提供了一种用于储能的新型多孔聚合物衍生的碳膜。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2018年第10期</span><b style="margin: 0 2px;">|</b><span>共10页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Luxin&option=202" target="_blank" rel="nofollow">Wang Luxin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ding Junjie&option=202" target="_blank" rel="nofollow">Ding Junjie;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sun Sai&option=202" target="_blank" rel="nofollow">Sun Sai;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Bin&option=202" target="_blank" rel="nofollow">Zhang Bin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tian Xiangyu&option=202" target="_blank" rel="nofollow">Tian Xiangyu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhu Jinhui&option=202" target="_blank" rel="nofollow">Zhu Jinhui;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Song Sannian&option=202" target="_blank" rel="nofollow">Song Sannian;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Bo&option=202" target="_blank" rel="nofollow">Liu Bo;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhuang Xiaodong&option=202" target="_blank" rel="nofollow">Zhuang Xiaodong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Yu&option=202" target="_blank" rel="nofollow">Chen Yu;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Key Lab for Advanced MaterialsEast China University of Science and TechnologyMeilong Road 130 200237 Shanghai China;</p> <p>Key Lab for Advanced MaterialsEast China University of Science and TechnologyMeilong Road 130 200237 Shanghai China;</p> <p>Key Lab for Advanced MaterialsEast China University of Science and TechnologyMeilong Road 130 200237 Shanghai China;</p> <p>Key Lab for Advanced MaterialsEast China University of Science and TechnologyMeilong Road 130 200237 Shanghai China;</p> <p>Key Lab for Advanced MaterialsEast China University of Science and TechnologyMeilong Road 130 200237 Shanghai China;</p> <p>The State Key Laboratory of Metal Matrix Composites and Shanghai Key Lab of Electrical Insulation and Thermal AgeingShanghai Jiao Tong UniversityDongchuan Road 800 200240 Shanghai China;</p> <p>State Key Laboratory of Functional Materials for InformaticsChinese Academy of SciencesChangning Road 865 200050 Shanghai China;</p> <p>School of ChemistrySuzhou University of Science and TechnologyNo. 1 Kerui Road 215009 Suzhou Jiangsu Province China;</p> <p>The State Key Laboratory of Metal Matrix Composites and Shanghai Key Lab of Electrical Insulation and Thermal AgeingShanghai Jiao Tong UniversityDongchuan Road 800 200240 Shanghai China;</p> <p>Key Lab for Advanced MaterialsEast China University of Science and TechnologyMeilong Road 130 200237 Shanghai China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=ionic porous polymer&option=203" rel="nofollow">ionic porous polymer;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=memristor&option=203" rel="nofollow">memristor;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=micro‐supercapacitor&option=203" rel="nofollow">micro‐supercapacitor;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=radical&option=203" rel="nofollow">radical;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=viologen&option=203" rel="nofollow">viologen;</a> </p> <div class="translation"> 机译：离子多孔聚合物;忆耳;微型超级电容器;激进;viologen; </div> </li> </ul> </div> </div> <div class="literature 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semiconductor polymer containing the composition, organic active layer containing the organic semiconductor polymer, organic thin film transistor containing the organic active layer, electronic device containing the organic thin film transistor and method of preparing the same</a> <b>[P]</b> . <span> 外国专利：  US8154016B2 </span> <span> . 2012-04-10</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：包含噻唑环的组合物，包含该组合物的有机半导体聚合物，包含该有机半导体聚合物的有机活性层，包含该有机活性层的有机薄膜晶体管，包含该有机薄膜晶体管的电子器件及其制备方法 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130425907887.html">Composition containing thiazole rings, organic semiconductor polymer containing the composition, organic active layer containing the organic semiconductor polymer, organic thin film transistor containing the organic active layer, electronic device containing the organic thin film transistor and method of preparing the same</a> <b>[P]</b> . <span> 外国专利：  US2011209762A1 </span> <span> . 2011-09-01</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：包含噻唑环的组合物，包含该组合物的有机半导体聚合物，包含有机半导体聚合物的有机活性层，包含有机活性层的有机薄膜晶体管，包含有机薄膜晶体管的电子器件及其制备方法 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130425638571.html">Composition containing thiazole rings, organic semiconductor polymer containing the composition, organic active layer containing the organic semiconductor polymer, organic thin film transistor containing the organic active layer, electronic device containing the organic thin film transistor and method of preparing the same</a> <b>[P]</b> . <span> 外国专利：  US8026369B2 </span> <span> . 2011-09-27</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：包含噻唑环的组合物，包含该组合物的有机半导体聚合物，包含有机半导体聚合物的有机活性层，包含有机活性层的有机薄膜晶体管，包含有机薄膜晶体管的电子器件及其制备方法 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704022435409','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img src="https://cdn.zhangqiaokeyan.com/img/loginclose.png" alt="关闭" onclick="$('.journalsub-pop-up').hide()"> <p class="pardon">抱歉，该期刊暂不可订阅，敬请期待！</p> <p 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