2D New Nonmetal Photocatalyst of Sulfur‐Doped h‐BN Nanosheeets with High Photocatalytic Activity

Zhao Gang; Wang Aizhu; He Weidong; Xing Yupeng; Xu Xijin

摘要

Abstract > 2D nonmetal hexagonal boron nitride nanosheets (h‐BNNS) are attracting more attention in the field of catalysis due to their excellent adsorption and photooxidation resistance performances. Here, for the first time, the possible adjustment of the bandgap of h‐BNNS (4.13 eV) by doping sulfur atoms is theoretically demonstrated and experimentally realized, which causes h‐BNNS (no photocatalytic property) to possess impressive visible light photocatalytic properties. The photodegradation efficiency (η) of S‐BNNS for rhodamine B reaches 97.2% for 3 h, and the photocatalytic hydrogen production efficiency is 1348.5 μmol h ?1 g ?1 , which are higher than those of the common visible light photocatalysts (S and g‐C <sub>3</sub> N <sub>4</sub> ). This approach is of guiding significance for the application of h‐BNNS in the field of photocatalysis. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 2D非金属六方硼氮化物纳米片（H-BNNS）由于其优异的吸附和光氧化抗性性能而在催化领域中吸引更多的注意。这里，首次通过掺杂硫原子的H-BNNS（4.13eV）的可能调节H-BNNS（4.13eV）的可能调节，并且实验地实现了H-BNN（无光催化性能）具有令人印象深刻的可见光光催化特性。罗丹明B的S-BNN的光降解效率（η）达到3小时的97.2％，光催化氢气生产效率为1348.5μmolH ？1 </ sup> G ？1 </ sup> ，这高于普通的可见光光催化剂（S和G-C） <sub> 3 </ sub> N. <sub> 4 </ sub> ）。这种方法是在光催化领域中施加H-BNN的指导意义。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2019年第7期</span><b style="margin: 0 2px;">|</b><span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhao Gang&option=202" target="_blank" rel="nofollow">Zhao Gang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Aizhu&option=202" target="_blank" rel="nofollow">Wang Aizhu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=He Weidong&option=202" target="_blank" rel="nofollow">He Weidong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xing Yupeng&option=202" target="_blank" rel="nofollow">Xing Yupeng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xu Xijin&option=202" target="_blank" rel="nofollow">Xu Xijin;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Laboratory of Functional Micro/Nano Materials and devicesUniversity of JinanJinan Shandong 250022 P. R. China;</p> <p>Laboratory of Functional Micro/Nano Materials and devicesUniversity of JinanJinan Shandong 250022 P. R. China;</p> <p>Laboratory of Functional Micro/Nano Materials and devicesUniversity of JinanJinan Shandong 250022 P. R. China;</p> <p>Laboratory of Functional Micro/Nano Materials and devicesUniversity of JinanJinan Shandong 250022 P. R. China;</p> <p>Laboratory of Functional Micro/Nano Materials and devicesUniversity of JinanJinan Shandong 250022 P. R. China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=2D material&option=203" rel="nofollow">2D material;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=density‐functional theory (DFT)&option=203" rel="nofollow">density‐functional theory (DFT);</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hydrogen evolution&option=203" rel="nofollow">hydrogen evolution;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nonmetal photocatalyst&option=203" rel="nofollow">nonmetal photocatalyst;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=sulfur‐doped h‐BN nanosheets&option=203" rel="nofollow">sulfur‐doped h‐BN nanosheets;</a> </p> <div class="translation"> 机译：2D材料;密度功能理论（DFT）;氢气进化;非金属光催化剂;硫磺掺杂的H-BN纳米液; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022434754.html">2D New Nonmetal Photocatalyst of Sulfur‐Doped h‐BN Nanosheeets with High Photocatalytic Activity</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhao Gang&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Zhao Gang,</a> <a 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href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=石康中&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,石康中</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=涂睿&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,涂睿</a> <span> <a href="/journal-cn-28399/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 催化学报 </a> </span> <span> . 2015</span><span>,第011期</span> </span> </div> </li> <li> <div> <b>6. </b><a class="enjiyixqcontent" href="/academic-conference-cn_meeting-9351_thesis/020222320793.html">新型Ag2O可见光光催化剂：自稳定性和高光催化活性</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=余火根&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 余火根</a> <span> <a href="/conference-cn-9351/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 第六届全国环境化学学术大会 </a> <span> <span> . 2011</span> </span> </div> </li> <li> <div> <b>7. </b><a 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METHOD</a> <b>[P]</b> . <span> 外国专利：  JP6408404B2 </span> <span> . 2018-10-17</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：光催化剂的组成，光催化活性的改进和光催化活性的改进方法 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130413343633.html">PHOTOCATALYST COMPOSITION, PHOTOCATALYTIC ACTIVITY IMPROVER AND PHOTOCATALYTIC ACTIVITY IMPROVING METHOD</a> <b>[P]</b> . <span> 外国专利：  JP2016172202A </span> <span> . 2016-09-29</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：光催化剂的组成，光催化活性的改进和光催化活性的改进方法 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130427311199.html">METHOD FOR PRODUCING A COMPOSITE CARBON NANOFIBER HAVING A PHOTOCATALYTIC ACTIVITY, COMPOSITE CARBON NANOFIBER HAVING A PHOTOCATALYTIC ACTIVITY PRODUCED BY THE METHOD, FILTER COMPRISING THE COMPOSITE CARBON NANOFIBER, AND THERMALLY STABLE PHOTOCATALYST SOL SOLUTION USED IN THE PRODUCTION METHOD</a> <b>[P]</b> . <span> 外国专利：  WO2010077011A2 </span> <span> . 2010-07-08</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：生产具有光催化活性的复合碳纳米纤维的方法，具有该方法生产的具有光催化活性的复合碳纳米纤维，包含复合碳纳米纤维和热稳定的光解产物的热分解碳纤维的方法 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" 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