Superior Energy Storage Performances of Polymer Nanocomposites via Modification of Filler/Polymer Interfaces

Zhang Xin; Li Bao‐Wen; Dong Lijie; Liu Hanxin; Chen Wen; Shen Yang; Nan Ce‐Wen

摘要

Abstract > Dielectric polymer nanocomposites by integration of high‐ E <sub>b</sub> polymer matrix and high‐ D (ε <sub>r</sub> ) ceramic fillers have shown great potential for dielectric and energy storage applications in modern electronic and electrical systems. Interface between ceramic fillers and polymer matrix is considered as a predominant factor to determine the dielectric performances of the nanocomposites. This review analyzes the influence of the interface on dielectric responses and breakdown strength in the nanocomposites, and discusses the viability of current interface engineering strategies in improving their energy storage capabilities. Two scopes of current interface modification approaches are focused from both structural and functional considerations in the dielectric ceramics/polymer nanocomposites: first, the organic/inorganic interface compatibility can be modified to generate homogeneous dispersion of ceramic nanoparticles in polymer matrix, which is the premise of fully realizing the synergistic combination of advantages of polymer and ceramic fillers; second, regulated local electrical and dielectric behaviors in interface region enable the enhancement of dielectric properties (both high dielectric constant and high breakdown strength) in resultant nanocomposites. In the last part, some present challenges and future perspectives are proposed to utilize the interface strategy for developing high energy density ceramics/polymer nanocomposites for dielectric and energy storage applications. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 介电聚合物纳米复合材料通过整合高 - e </ i> <sub> b </ sub> 聚合物基质和高 - d </ i> （ε. <sub> r </ sub> ）陶瓷填充物在现代电子和电气系统中显示了介电和能量存储应用的巨大潜力。陶瓷填料和聚合物基质之间的界面被认为是确定纳米复合材料的介电性能的主要因素。该综述分析了界面对纳米复合材料中介电响应和击穿强度的影响，并探讨了当前界面工程策略的可行性，提高了能量存储能力。电流界面修改方法的两个范围从介电陶瓷/聚合物纳米复合材料中的结构和功能考虑都集中起来：首先，可以改变有机/无机界面相容性以在聚合物基质中产生陶瓷纳米颗粒的均匀分散，这是前提完全实现聚合物和陶瓷填料的共同组合;界面区域中的第二，局部局部电气和介电行为能够在所得到的纳米复合材料中提高介电性质（两种高介电常数和高击穿强度）。在最后，提出了一些存在的挑战和未来的观点，以利用用于开发高能密度陶瓷/聚合物纳米复合材料的界面策略，用于介电和能量储存应用。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2018年第11期</span><b style="margin: 0 2px;">|</b><span>共28页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Xin&option=202" target="_blank" rel="nofollow">Zhang Xin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Bao‐Wen&option=202" target="_blank" rel="nofollow">Li Bao‐Wen;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dong Lijie&option=202" target="_blank" rel="nofollow">Dong Lijie;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Hanxin&option=202" target="_blank" rel="nofollow">Liu Hanxin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Wen&option=202" target="_blank" rel="nofollow">Chen Wen;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Shen Yang&option=202" target="_blank" rel="nofollow">Shen Yang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Nan Ce‐Wen&option=202" target="_blank" rel="nofollow">Nan Ce‐Wen;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Center of Smart Materials and DevicesWuhan University of TechnologyWuhan 430070 China;</p> <p>Center of Smart Materials and DevicesWuhan University of TechnologyWuhan 430070 China;</p> <p>Center of Smart Materials and DevicesWuhan University of TechnologyWuhan 430070 China;</p> <p>Center of Smart Materials and DevicesWuhan University of TechnologyWuhan 430070 China;</p> <p>Center of Smart Materials and DevicesWuhan University of TechnologyWuhan 430070 China;</p> <p>School of Materials Science and EngineeringTsinghua UniversityBeijing 100084 China;</p> <p>Center of Smart Materials and DevicesWuhan University of TechnologyWuhan 430070 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=dielectric&option=203" rel="nofollow">dielectric;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=energy storage&option=203" rel="nofollow">energy storage;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=interfaces&option=203" rel="nofollow">interfaces;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanoparticles&option=203" rel="nofollow">nanoparticles;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=polymer nanocomposites&option=203" rel="nofollow">polymer nanocomposites;</a> </p> <div class="translation"> 机译：电介质;储能;界面;纳米颗粒;聚合物纳米复合材料; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022434627.html">Superior Energy Storage Performances of Polymer Nanocomposites via Modification of Filler/Polymer Interfaces</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Xin&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Zhang Xin,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Bao‐Wen&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Li Bao‐Wen,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dong Lijie&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Dong Lijie,</a> <a href="/journal-foreign-18063/" target="_blank" rel="nofollow" class="tuijian_authcolor">Advanced materials interfaces .</a> <span>2018</span><span>,第11期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：通过改性填料/聚合物界面的高储能性能</span> </p> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704028354706.html">Ultrahigh energy storage performance of a polymer-based nanocomposite via interface engineering</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Peng&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Wang Peng,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Pan Zhongbin&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Pan Zhongbin,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Weilin&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Wang Weilin,</a> <a href="/journal-foreign-35176/" target="_blank" rel="nofollow" class="tuijian_authcolor">Journal of Materials Chemistry, A. 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