Rational Design of Fe        <sub >1?</sub>1?        <i >          <sub>x</sub>                  <sub >x</sub>x                S/Fe        <sub >3</sub>3        O        <sub >4</sub>4        /Nitrogen and Sulfur‐Doped Porous Carbon with Enhanced Oxygen Reduction Reaction Catalytic Activity

Zhang Juewen; Xu Dan; Wang Cancan; Guo Jiangna; Yan Feng

摘要

Abstract > In this paper, the rational design of Fe‐N‐, Fe‐S‐, and Fe‐N‐S‐based model catalysts for oxygen reduction reaction (ORR), developed using task‐specific hypercrosslinked polymers as precursors is presented. Based on the model catalysts, atom‐induced differences in ORR performance are carefully examined. In the S‐doped carbons, Fe <sub>1?</sub> <sub>x</sub> S forms the metal nanoparticles, while the N sourced together with FeCl <sub>3</sub> ensures the uniform distribution of Fe <sub>3</sub> O <sub>4</sub> . Obtained results indicate that N/Fe <sub>3</sub> O <sub>4</sub> acts as the higher catalytic active site, whereas the S/Fe <sub>1?</sub> <sub>x</sub> S deteriorates the ORR catalytic activity. However, due to the synergistic effect between Fe <sub>1?</sub> <sub>x</sub> S /Fe <sub>3</sub> O <sub>4</sub> and N, the S‐doped carbons can substantially enhance the ORR performance. Hence, this work provides guidance for the efficient design of Fe‐N‐S‐based catalysts for ORR. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 本文介绍了使用任务特异性高速链接聚合物作为前体的氧还原反应（ORR）的Fe-N-，Fe-S和Fe-N-S基催化剂的合理设计。基于模型催化剂，仔细检查原子诱导的ORR性能差异。在S掺杂的碳碳水化合物中 <sub> 1？</ sub> <sub> x </ sub> </ i> S形成金属纳米颗粒，而n与fecl一起源 <sub> 3 </ sub> 确保Fe的统一分配 <sub> 3 </ sub> O. <sub> 4 </ sub> 。获得的结果表明N / FE <sub> 3 </ sub> O. <sub> 4 </ sub> 作为更高的催化活性位点，而S / Fe <sub> 1？</ sub> <sub> x </ sub> </ i> S劣化了ORR催化活性。但是，由于FE之间的协同效应 <sub> 1？</ sub> <sub> x </ sub> </ i> S / FE. <sub> 3 </ sub> O. <sub> 4 </ sub> 并且，S掺杂的碳基本上可以大大提高ORR性能。因此，这项工作为ORR的Fe-N-S基催化剂的有效设计提供了指导。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2018年第7期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Juewen&option=202" target="_blank" rel="nofollow">Zhang Juewen;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xu Dan&option=202" target="_blank" rel="nofollow">Xu Dan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Cancan&option=202" target="_blank" rel="nofollow">Wang Cancan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Guo Jiangna&option=202" target="_blank" rel="nofollow">Guo Jiangna;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yan Feng&option=202" target="_blank" rel="nofollow">Yan Feng;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Jiangsu Key Laboratory of Advanced Functional Polymer Design and ApplicationSoochow UniversitySuzhou 215123 China;</p> <p>Jiangsu Key Laboratory of Advanced Functional Polymer Design and ApplicationSoochow UniversitySuzhou 215123 China;</p> <p>Jiangsu Key Laboratory of Advanced Functional Polymer Design and ApplicationSoochow UniversitySuzhou 215123 China;</p> <p>Jiangsu Key Laboratory of Advanced Functional Polymer Design and ApplicationSoochow UniversitySuzhou 215123 China;</p> <p>Jiangsu Key Laboratory of Advanced Functional Polymer Design and ApplicationSoochow UniversitySuzhou 215123 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=electrocatalysis&option=203" rel="nofollow">electrocatalysis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=heteroatom&option=203" rel="nofollow">heteroatom;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hypercrosslinked polymers&option=203" rel="nofollow">hypercrosslinked polymers;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=oxygen reduction&option=203" rel="nofollow">oxygen reduction;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=porous carbon&option=203" rel="nofollow">porous carbon;</a> </p> <div class="translation"> 机译：电催化;杂原子;超交联的聚合物;氧气减少;多孔碳; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/academic-journal-cn_transactions-nonferrous-metals-society-china_thesis/0201289457064.html">用于氧还原反应的氮掺杂空心多孔碳球封装的过渡金属氮化物的制备和性能</a> <b>[J]</b> . 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Rational Design of Fe 1?1? x xx S/Fe 33 O 44 /Nitrogen and Sulfur‐Doped Porous Carbon with Enhanced Oxygen Reduction Reaction Catalytic Activity

摘要

Rational Design of Fe _1?1? _x _xx S/Fe ₃3 O ₄4 /Nitrogen and Sulfur‐Doped Porous Carbon with Enhanced Oxygen Reduction Reaction Catalytic Activity