Mussel‐Inspired Polyesters with Aliphatic Pendant Groups Demonstrate the Importance of Hydrophobicity in Underwater Adhesion

Xu Ying; Liu Qianhui; Narayanan Amal; Jain Dharamdeep; Dhinojwala Ali; Joy Abraham

摘要

Abstract > Recognizing the potential for synthetic adhesives that can function in wet environments, elements of mussel foot proteins such as L ‐3,4‐dihydroxyphenylalanine (DOPA) and phosphoserine have been incorporated into synthetic adhesives. Such adhesives have corroborated the advantage of surface active groups like DOPA, but have not yet demonstrated superior performance in wet or underwater environments, without using organic solvents. What has been conspicuously absent from such designs is the effect of hydrophobic components in the performance of underwater adhesives. Herein it is shown that incorporation of hydrophobic groups in low modulus polyester adhesives provides very high lap‐shear strength and resistance to water penetration. In addition to the excellent performance in wet conditions, the designed adhesive can be applied underwater without any solvent, is biodegradable, and is designed from soybean oil, which is a readily available and renewable resource. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 识别可以在潮湿环境中起作用的合成粘合剂的潜力，贻贝脚蛋白的元素如 l </ i> -3,4-二羟基苯丙氨酸（DOPA）和磷素已掺入合成粘合剂中。这种粘合剂已经证实了像多脂一样的表面活性基团的优点，但尚未在潮湿或水下环境中表现出优异的性能，而不使用有机溶剂。这种设计显着缺席的是疏水成分在水下粘合剂的性能方面的影响。在此显示，在低模量聚酯粘合剂中掺入疏水基团提供非常高的搭接剪切强度和与水渗透的抗性。除了在潮湿条件下的优异性能之外，设计的粘合剂可以在水下施加无任何溶剂，是可生物降解的，并且由大豆油设计，这是一种易于可获得和可再生的资源。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2017年第22期</span><b style="margin: 0 2px;">|</b><span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xu Ying&option=202" target="_blank" rel="nofollow">Xu Ying;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Qianhui&option=202" target="_blank" rel="nofollow">Liu Qianhui;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Narayanan Amal&option=202" target="_blank" rel="nofollow">Narayanan Amal;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jain Dharamdeep&option=202" target="_blank" rel="nofollow">Jain Dharamdeep;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dhinojwala Ali&option=202" target="_blank" rel="nofollow">Dhinojwala Ali;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Joy Abraham&option=202" target="_blank" rel="nofollow">Joy Abraham;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Polymer ScienceThe University of AkronAkron OH 44325 USA;</p> <p>Department of Polymer ScienceThe University of AkronAkron OH 44325 USA;</p> <p>Department of Polymer ScienceThe University of AkronAkron OH 44325 USA;</p> <p>Department of Polymer ScienceThe University of AkronAkron OH 44325 USA;</p> <p>Department of Polymer ScienceThe University of AkronAkron OH 44325 USA;</p> <p>Department of Polymer ScienceThe University of AkronAkron OH 44325 USA;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=catechol polymers&option=203" rel="nofollow">catechol polymers;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=DOPA polymers&option=203" rel="nofollow">DOPA polymers;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=mussel inspired adhesives&option=203" rel="nofollow">mussel inspired adhesives;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=synthetic polyester adhesives&option=203" rel="nofollow">synthetic polyester adhesives;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=underwater hydrophobic polyester adhesives&option=203" rel="nofollow">underwater hydrophobic polyester adhesives;</a> </p> <div class="translation"> 机译：儿茶酚聚合物;多巴聚合物;贻贝启发粘合剂;合成聚酯粘合剂;水下疏水性聚酯粘合剂; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022433645.html">Mussel‐Inspired Polyesters with Aliphatic Pendant Groups Demonstrate the Importance of Hydrophobicity in Underwater Adhesion</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xu Ying&option=202" target="_blank" rel="nofollow" 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href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=马前&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 马前</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=雷科文&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,雷科文</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=俞麟&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,俞麟</a> <span> <a href="/conference-cn-43337/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 2017中国生物材料大会 </a> <span> <span> . 2017</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020311522668.html">脂肪族聚酯生物材料的亲水性增强改性研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=姜元芹&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 姜元芹</a> <span> . 2013</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120479423.html">脂族聚酯树脂组合物和脂族聚酯树脂成型体以及脂族聚脂树脂成型体的制造方法</a> <b>[P]</b> . <span> 中国专利： CN100480327C </span> <span> . 2009.04.22</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120105116395.html">脂族聚酯树脂组合物和脂族聚酯树脂成型体以及脂族聚脂树脂成型体的制造方法</a> <b>[P]</b> . <span> 中国专利： CN1910236A </span> <span> . 2007-02-07</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130412084012.html">AMPHIPHILIC COPOLYMERS COMPRISING HYDROPHILIC BACKBONE WITH PENDANT ALIPHATIC GROUPS AS HYDROPHOBIC COMPONENT</a> <b>[P]</b> . <span> 外国专利：  IN276754B </span> <span> . 2016-11-04</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：包含亲水主链与侧链脂族基团作为疏水性组分的两性共聚物 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130422892735.html">(54) Title: UV ABSORBING COMPLEX POLYESTER POLYMERS, COMPOSITIONS CONTAINING UV ABSORBING COMPLEX POLYESTER POLYMERS, AND RELATED METHODS (57) Abstract: A UV absorbing complex polyol polyester polymer is the product of a reaction scheme that includes: (i) the esterification of a polyol and a dianhydride, wherein the esterification is carried out under conditions that facilitate substantially only anhydride opening, to form a polyester polymer comprising at least two pendant carboxylic groups, and at least two hy-droxyl groups: and (ii) the reaction of at least one pendant carboxylic group and at least one terminal hydroxyl group of the polyester polymer with an epoxide having a functional group, wherein the epoxide comprises an UV absorbing moiety. A crosslinked UV absorbing complex polyol polyester polymer that is reaction product of a random copolyesterification esterification reaction and/or the esterification product.</a> <b>[P]</b> . <span> 外国专利：  IN2012MN01234A </span> <span> . 2012-08-24</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：（54）标题：吸收紫外线的复合聚酯聚合物，包含紫外线吸收的复合聚酯聚合物的组成及相关方法（57）摘要：吸收紫外线的复合多元醇聚酯聚合物是反应方案的产物，该反应方案包括：（i）酯化多元醇和二酐，其中所述酯化反应在基本上仅促进酸酐开放的条件下进行，以形成包含至少两个侧基羧基和至少两个羟基的聚酯聚合物：和（ii）具有具有官能团的环氧化物的聚酯聚合物的至少一个侧链羧基和至少一个末端羟基，其中该环氧化物包含UV吸收部分。交联的吸收紫外线的复合多元醇聚酯聚合物，它是无规共聚酯化酯化反应和/或酯化产物的反应产物。 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130460775724.html">POLYIMIDE/ALIPHATIC POLYESTER COPOLYMER WITHOUT PENDANT CARBOXYLIC ACID GROUP</a> <b>[P]</b> . <span> 外国专利：  JPH06200029A </span> <span> . 1994-07-19</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：无侧链羧酸基团的聚酰亚胺/脂肪族聚酯共聚物 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704022433645','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img src="https://cdn.zhangqiaokeyan.com/img/loginclose.png" alt="关闭" onclick="$('.journalsub-pop-up').hide()"> <p class="pardon">抱歉，该期刊暂不可订阅，敬请期待！</p> <p 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