Behavior of Alkaline‐Metal Catalysts in Supercritical Water Gasification of Lignite

机译：碱金属催化剂在褐煤超临界水气化中的行为

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Abstract > The efficient utilization of abundant low‐rank coals, which show high moisture and ash content, is significant for coal‐based energy systems. The gasification of Zhaotong lignite was performed with different alkaline‐metal catalysts, such as KOH, NaOH, K <sub>2</sub> CO <sub>3</sub> , and Na <sub>2</sub> CO <sub>3</sub> , in supercritical water. The behavior of the alkaline metal was also investigated. Potassium shows better catalytic activity than sodium. KOH not only promotes breakage of chemical bonds in the coal matrix to generate low‐molecular‐weight gases, but also alters the pore structure of the char to improve the gasification of carbon in the residue. However, potassium is partly inactivated upon reaction with minerals in coal in supercritical water gasification. In situ protection of potassium is realized by adding Ca(OH) <sub>2</sub> under supercritical conditions. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <标题类型=“main”>抽象</ title> > 对于煤基能量系统，有效利用丰富的低级煤，其显示出高的水分和灰分含量。 Zhaotong Lignite的气化用不同的碱金属催化剂进行，例如KOH，NaOH，K. <sub> 2 </ sub> CO. <sub> 3 </ sub> 和na <sub> 2 </ sub> CO. <sub> 3 </ sub> ，在超临界水中。还研究了碱金属的行为。钾显示比钠的催化活性更好。 KOH不仅促进了煤基质中的化学键的破损，以产生低分子量气体，而且还改变了焦炭的孔结构以改善残留物中碳的气化。然而，在超临界水气化中的煤中的矿物反应后部分地失活。通过添加CA（OH）实现原位保护钾 <sub> 2 </ sub> 在超临界条件下。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16566/'>《Chemical Engineering & Technology: Industrial Chemistry -Plant Equipment -Process Engineering -Biotechnology》</a> <b style="margin: 0 2px;">|</b><span>2018年第8期</span><b style="margin: 0 2px;">|</b><span>共8页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Qu Xuan&option=202" target="_blank" rel="nofollow">Qu Xuan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhou Xianxian&option=202" target="_blank" rel="nofollow">Zhou Xianxian;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yan Xiaoqiang&option=202" target="_blank" rel="nofollow">Yan Xiaoqiang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Rong&option=202" target="_blank" rel="nofollow">Zhang Rong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Bi Jicheng&option=202" target="_blank" rel="nofollow">Bi Jicheng;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Institute of Coal ChemistryChinese Academy of Sciences27 South Taoyuan Road 030001 Taiyuan Shanxi China;</p> <p>Taiyuan University of TechnologyNo. 79 West Yingze Street 030024 Taiyuan Shanxi China;</p> <p>Institute of Coal ChemistryChinese Academy of Sciences27 South Taoyuan Road 030001 Taiyuan Shanxi China;</p> <p>Institute of Coal ChemistryChinese Academy of Sciences27 South Taoyuan Road 030001 Taiyuan Shanxi China;</p> <p>Institute of Coal ChemistryChinese Academy of Sciences27 South Taoyuan Road 030001 Taiyuan Shanxi China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/238.html" title="化学工业">化学工业;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Alkaline‐metal catalysts&option=203" rel="nofollow">Alkaline‐metal catalysts;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lignite&option=203" rel="nofollow">Lignite;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Low‐rank coals&option=203" rel="nofollow">Low‐rank coals;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Supercritical water gasification&option=203" rel="nofollow">Supercritical water gasification;</a> </p> <div class="translation"> 机译：碱金属催化剂;褐煤;低级煤;超临界水气化; </div> </li> <li> <span class="lefttit">入库时间</span> <span>2022-08-19 23:50:26</span> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022180841.html">Behavior of Alkaline‐Metal Catalysts in Supercritical Water Gasification of Lignite</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Qu Xuan&option=202" target="_blank" rel="nofollow" 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