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首页> 外文期刊>ChemSusChem >Origins of Catalyst Inhibition in the Manganese‐Catalysed Oxidation of Lignin Model Compounds with H2O2
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Origins of Catalyst Inhibition in the Manganese‐Catalysed Oxidation of Lignin Model Compounds with H2O2

机译：催化剂抑制在锰催化的木质素模型化合物与H2O2中的氧化

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Abstract > The upgrading of complex bio‐renewable feedstock, such as lignocellulose, through depolymerisation benefits from the selective reactions at key functional groups. Applying homogeneous catalysts developed for selective organic oxidative transformations to complex feedstock such as lignin is challenged by the presence of interfering components. The selection of appropriate model compounds is essential in applying new catalytic systems and identifying such interferences. Here, it was shown by using as an example the oxidation of a model substrate containing a β‐O‐4 linkage with H <sub>2</sub> O <sub>2</sub> and an in?situ‐prepared manganese‐based catalyst, capable of efficient oxidation of benzylic alcohols, that interference from compounds liberated during the reaction can prevent its application to lignocellulose depolymerisation. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 通过在关键官能团的选择性反应中升级木质可再生原料（如木质纤维素）的改善。通过干扰组分的存在，将开发用于选择性有机氧化转化为复合原料的复杂原料的均相催化剂施加到复杂的原料中。选择适当的模型化合物对于应用新的催化系统并识别这种干扰是必要的。在此，通过用作含有β-O-4连杆的模型衬底的氧化来显示含有H与H的示例 <sub> 2 </ sub> O. <sub> 2 </ sub> 并且在α原位制备的锰基催化剂，能够有效氧化苄醇，从反应过程中释放的化合物的干扰可以防止其在木质纤维素解聚中的应用。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16185/'>《ChemSusChem》</a> <b style="margin: 0 2px;">|</b><span>2019年第13期</span><b style="margin: 0 2px;">|</b><span>共8页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Barbieri Alessia&option=202" target="_blank" rel="nofollow">Barbieri Alessia;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kasper Johann B.&option=202" target="_blank" rel="nofollow">Kasper Johann B.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Mecozzi Francesco&option=202" target="_blank" rel="nofollow">Mecozzi Francesco;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lanzalunga Osvaldo&option=202" target="_blank" rel="nofollow">Lanzalunga Osvaldo;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Browne Wesley R.&option=202" target="_blank" rel="nofollow">Browne Wesley R.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Dipartimento di ChimicaUniversita'di Roma “La Sapienza”P.le A. Moro 5 I-00185 Rome Italy;</p> <p>Molecular Inorganic ChemistryUniversity of GroningenNijenborgh 4 9747AG Groningen The Netherlands;</p> <p>Molecular Inorganic ChemistryUniversity of GroningenNijenborgh 4 9747AG Groningen The Netherlands;</p> <p>Dipartimento di ChimicaUniversita'di Roma “La Sapienza”P.le A. Moro 5 I-00185 Rome Italy;</p> <p>Molecular Inorganic ChemistryUniversity of GroningenNijenborgh 4 9747AG Groningen The Netherlands;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/159.html" title="化学">化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=catalysis&option=203" rel="nofollow">catalysis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=inhibition&option=203" rel="nofollow">inhibition;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=lignin&option=203" rel="nofollow">lignin;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=manganese&option=203" rel="nofollow">manganese;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=oxidation&option=203" rel="nofollow">oxidation;</a> </p> <div class="translation"> 机译：催化;抑制;木质素;锰;氧化; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022092996.html">Origins of Catalyst Inhibition in the Manganese‐Catalysed Oxidation of Lignin Model Compounds with H2O2</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Barbieri Alessia&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Barbieri Alessia,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kasper Johann 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<span>机译：在紫外线辐射下通过控制性光催化氧化与二氧化钛纳米催化剂从含酚木质素模型化合物的废水中生产短链脂肪酸的方法和方法 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130425995367.html">Method and process of producing short chain fatty acids from waste stream containing phenolic lignin model compounds by controlled photocatalytic oxidation with titanium dioxide nanocatalyst in the presence of ultraviolet radiation</a> <b>[P]</b> . <span> 外国专利： <!-- 美国专利： --> US2011084231A1 </span> <span> . 2011-04-14</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：在紫外线辐射下通过二氧化钛纳米催化剂的可控光催化氧化从含酚木质素模型化合物的废料流中生产短链脂肪酸的方法和方法 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130434546115.html">USE OF METAL COMPLEX COMPOUNDS COMPRISING PYRIDINE PYRIMIDINE OR S-TRIAZINE DERIVED LIGANDS AS CATALYSTS FOR OXIDATIONS WITH ORGANIC PEROXY ACIDS AND/OR PRECURSORS OF ORGANIC PEROXY ACID AND H2O2</a> <b>[P]</b> . <span> 外国专利： <!-- 韩国专利： --> KR20060126531A </span> <span> . 2006-12-07</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：包含吡啶嘧啶或S-三嗪衍生的配位体的金属络合物作为催化剂用于氧化有机高纯酸和/或有机高纯酸和H2O2的前体 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704022092996','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div 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