Fabrication of Core‐Shell Ni2P@N, P?Co‐Doped Carbon/Reduced Graphene Oxide Composite as Anode Material for Lithium‐ and Sodium‐Ion Batteries

Li Yongsheng; Zhang Jianmin; Li Dan; Ding Jie; Liu Yushan; Cai Qiang

摘要

Abstract > Commonly, carbon layer was a suitable choice to enhance the conductivity and reduce the large volume effect of Ni <sub>2</sub> P nanoparticles (NPs) in electrochemical applications. The doped nitrogen (N) and phosphorous (P) atoms in carbon could further improve its performance. In this paper, core‐shell structure Ni <sub>2</sub> P@N, P‐co‐doped carbon (Ni <sub>2</sub> P@N, P?C) NPs were loaded onto reduced graphene oxide nanosheets (GN) to form new composite serial Ni <sub>2</sub> P@N, P?C/GN, which was designed for the combination of these merits and successfully obtained by two‐step method (firstly hydrothermal process and secondly phosphorization process). As anodes for LIBs and SIBs, the responding electrochemical studies showed the Ni <sub>2</sub> P@N, P?C/GN‐0.4 electrode exhibited an outstanding specific capacity of 450?mA?h?g ?1 at 5?A?g ?1 after 2000 cycles in lithium‐ion batteries (LIBs) and maintained 110?mA?h?g ?1 at 2?A?g ?1 after 3000 cycles in sodium‐ion batteries (SIBs), respectively. These results showed that Ni <sub>2</sub> P@N, P?C/GN material could be an excellent candidate for energy storage area. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 通常，碳层是增强导电性并降低Ni的大体积效果的合适选择 <sub> 2 </ sub> 电化学应用中的P纳米颗粒（NPS）。碳中掺杂的氮气（N）和磷（P）原子可以进一步提高其性能。本文核心壳结构NI <sub> 2 </ sub> p @ n，p-掺杂碳（ni <sub> 2 </ sub> p @ n，p≤c）nps加载到氧化石墨烯纳米片（Gn）上以形成新的复合串行ni <sub> 2 </ sub> P @ n，p？c / gn，其设计用于这些优点的组合，并通过两步法（首先水热过程和第二磷化过程）成功获得。作为LIBS和SIBS的阳极，响应的电化学研究显示了NI <sub> 2 </ sub> p @ n，p？c / gn-0.4电极表现出450？ma？h？g的出色特定容量？1 </ sup> 在5？a？g ？1 </ sup> 在锂离子电池（LIBS）中2000次循环后，保持110？MA？H？G. ？1 </ sup> 在2？a？g ？1 </ sup> 在钠离子电池（SIBS）中3000次循环后。这些结果表明ni <sub> 2 </ sub> P @ N，P？C / GN材料可以是能量存储区域的优异候选者。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16042/'>《ChemElectroChem》</a> <b style="margin: 0 2px;">|</b><span>2019年第21期</span><b style="margin: 0 2px;">|</b><span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Yongsheng&option=202" target="_blank" rel="nofollow">Li Yongsheng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Jianmin&option=202" target="_blank" rel="nofollow">Zhang Jianmin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Dan&option=202" target="_blank" rel="nofollow">Li Dan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ding Jie&option=202" target="_blank" rel="nofollow">Ding Jie;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Yushan&option=202" target="_blank" rel="nofollow">Liu Yushan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cai Qiang&option=202" target="_blank" rel="nofollow">Cai Qiang;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>College of ChemistryZhengzhou UniversityZhengzhou 450001 PR China;</p> <p>College of ChemistryZhengzhou UniversityZhengzhou 450001 PR China;</p> <p>College of ChemistryZhengzhou UniversityZhengzhou 450001 PR China;</p> <p>College of ChemistryZhengzhou UniversityZhengzhou 450001 PR China;</p> <p>College of ChemistryZhengzhou UniversityZhengzhou 450001 PR China;</p> <p>Key Laboratory for Advanced Materials of Ministry of Education and College of Materials Science and EngineeringTsinghua UniversityBeijing 100084 PR China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=dinickel phosphide&option=203" rel="nofollow">dinickel phosphide;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=core-shell&option=203" rel="nofollow">core-shell;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=doping&option=203" rel="nofollow">doping;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=lithium-ion batteries&option=203" rel="nofollow">lithium-ion batteries;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=sodium-ion batteries.&option=203" rel="nofollow">sodium-ion batteries.;</a> </p> <div class="translation"> 机译：DINICKEL磷化物;核心壳;掺杂;锂离子电池;钠离子电池。; 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