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Red Phosphorus/Onion‐like Mesoporous Carbon Composite as High‐Performance Anode for Sodium‐Ion Battery

机译：红磷/洋葱状介孔碳复合材料作为钠离子电池的高性能阳极

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Abstract > Red phosphorus has been regarded as an attractive candidate for the anode of sodium‐ion batteries (NIBs) because it delivers a high theoretical capacity (2596?mAh?g ?1 ) at low potentials. However, the electrochemical performances of red P are still not satisfactory for viable applications mainly due to its intrinsic low conductivity and large volume swelling associated with sodiation reactions. Here, we develop onion‐like mesoporous carbon nanoparticles (OCNPs) to serve as conductive host for red P. The OCNPs can alleviate the large volume swelling of red P, and allow the fast electron and Na + transport. The resulting P/OCNPs composite electrode achieves excellent rate performance of 1286.7?mAh?g ?1 at 2?C, and retained discharge capacity of 1057.5?mAh?g ?1 after 150 cycles at 0.5?C. The improved stability of the composite electrode is also confirmed by the structure integrity after the cycling test. Our work presents a feasible approach to address the challenges of red P for high‐capacity anode of NIBs. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 红磷被认为是钠离子电池（尖端）阳极的有吸引力的候选者，因为它提供了高理论能力（2596？MAH？G. ？1 </ sup> ）在低潜力。然而，对于可行的应用，红色P的电化学性能仍然是不令人满意的，主要是由于其内在的低导电性和与调解反应相关的大体积膨胀。在这里，我们培养洋葱的中孔碳纳米粒子（OCNP）用作红色P的导电宿主。OCNP可以缓解红色P的大体积肿胀，并允许快速电子和NA + </ sup> 运输。所得到的P / OCNPS复合电极实现优异的速率性能为1286.7？MAH？G. ？1 </ sup> 在2？c，并保留放电容量为1057.5？mah？g ？1 </ sup> 在0.5℃下150次循环后。通过循环试验后的结构完整性也证实了复合电极的改善稳定性。我们的工作提出了一种可行的方法来解决红色P对NIB的高容量阳极的挑战。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16042/'>《ChemElectroChem》</a> <b style="margin: 0 2px;">|</b><span>2019年第22期</span><b style="margin: 0 2px;">|</b><span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liang Xiaoqiang&option=202" target="_blank" rel="nofollow">Liang Xiaoqiang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chang Caiyun&option=202" target="_blank" rel="nofollow">Chang Caiyun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Guo Wenbin&option=202" target="_blank" rel="nofollow">Guo Wenbin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jiang Xingmao&option=202" target="_blank" rel="nofollow">Jiang Xingmao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xiong Chunyan&option=202" target="_blank" rel="nofollow">Xiong Chunyan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Pu Xiong&option=202" target="_blank" rel="nofollow">Pu Xiong;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>CAS Center for Excellence in Nanoscience Beijing Key Laboratory of Micro-nano Energy and Sensor Beijing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBeijing 100083 China;</p> <p>CAS Center for Excellence in Nanoscience Beijing Key Laboratory of Micro-nano Energy and Sensor Beijing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBeijing 100083 China;</p> <p>CAS Center for Excellence in Nanoscience Beijing Key Laboratory of Micro-nano Energy and Sensor Beijing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBeijing 100083 China;</p> <p>Hubei Provincial Research Center of Engineering and Technology for New Energy Material Key Laboratory for Green Chemical Process of Ministry of Education School of Chemical Engineering &</p> <p>PharmacyWuhan Institute of TechnologyWuhan 430205 China;</p> <p>Hubei Provincial Research Center of Engineering and Technology for New Energy Material Key Laboratory for Green Chemical Process of Ministry of Education School of Chemical Engineering &</p> <p>PharmacyWuhan Institute of TechnologyWuhan 430205 China;</p> <p>CAS Center for Excellence in Nanoscience Beijing Key Laboratory of Micro-nano Energy and Sensor Beijing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBeijing 100083 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=red phosphorus&option=203" rel="nofollow">red phosphorus;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=sodium-ion battery&option=203" rel="nofollow">sodium-ion battery;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=mesoporous carbon&option=203" rel="nofollow">mesoporous carbon;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=anode&option=203" rel="nofollow">anode;</a> </p> <div class="translation"> 机译：红磷;钠离子电池;中孔碳;阳极; </div> </li> <li> <span class="lefttit">入库时间</span> <span>2022-08-19 23:30:10</span> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022060487.html">Red Phosphorus/Onion‐like Mesoporous Carbon Composite as High‐Performance Anode for Sodium‐Ion Battery</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liang Xiaoqiang&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Liang Xiaoqiang,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chang Caiyun&option=202" target="_blank" rel="nofollow" class="tuijian_auth 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href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=许并社&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,许并社</a> <span> <a href="/conference-cn-20177/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 第八届全国新型炭材料学术研讨会 </a> <span> <span> . 2007</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020314617056.html">石墨烯复合二氧化锡和红磷的制备及其钠离子电池性能研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=裴龙凯&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 裴龙凯</a> <span> . 2015</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/061204118401.html">一种掺氟碳包覆的磷酸焦磷酸铁钠@介孔碳复合材料及其制备和在钠离子电池中的应用</a> <b>[P]</b> . <span> 中国专利： CN110061233B </span> <span> . 2020.11.24</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120103855174.html">一种氮掺杂碳包覆的磷酸铬锰钠@介孔碳复合材料及其制备方法和在钠离子电池中的应用</a> <b>[P]</b> . <span> 中国专利： CN111224085A </span> <span> . 2020-06-02</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130431476112.html">METHOD FOR PREPARING BLACK PHOSPHORUS OR BLACK PHOSPHORUS-CARBON COMPOSITE, PREPARED BLACK PHOSPHORUS AND BLACK PHOSPHORUS-CARBON COMPOSITE, LITHIUM RECHARGEABLE BATTERY COMPRISING THE BLACK PHOSPHORUS-CARBON COMPOSITE, AND METHOD FOR USING THE RECHARGEABLE BATTERY</a> <b>[P]</b> . <span> 外国专利：  JP2009184861A </span> <span> . 2009-08-20</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：制备黑色磷或黑色磷碳复合材料的方法，制备的黑色磷和黑色磷碳复合材料，包括黑色磷碳复合材料的锂可充电电池以及使用可充电电池的方法 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130431976778.html">METHOD FOR PREPARING BLACK PHOSPHORUS AND 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auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：制备黑磷或黑磷碳复合物的方法，包括制备的黑磷或黑磷碳复合物的锂可充电电池以及使用该可充电电池的方法 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704022060487','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img src="https://cdn.zhangqiaokeyan.com/img/loginclose.png" alt="" onclick="$('.journalsub-pop-up').hide()"> <p class="pardon">抱歉，该期刊暂不可订阅，敬请期待！</p> <p 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