Effect of the Structure and Mesoporosity in Ni/Zeolite Catalysts for        <i >nn        ‐Hexadecane Hydroisomerisation and Hydrocracking

摘要

Abstract >The hydroisomerisation/hydrocracking properties of Ni‐zeolite catalysts (H‐MFI and H‐Beta) are studied using n‐hexadecane as model compound and compared with those of Ni/ASA (amorphous silica‐alumina) as reference catalyst. In the case of H‐Beta, the effect of the introduction of mesoporosity by controlled desilication is also investigated. The results indicate that Ni on desilicated H‐Beta catalysts shows very interesting characteristics for the potential use in the production of biofuel from vegetable/algal oil, or the upgrading of biomass‐derived Fischer–Tropsch waxes. Ni/H‐Beta shows lower activity with respect to Ni/H‐MFI, but significantly lower formation of gases and much better hydroisomerisation activity. The introduction of mesoporosity by desilication enhances the activity, while still maintaining an acceptable gas formation and good hydroisomerisation properties. Furthermore, the desilication treatment improves the stability with respect to carbon formation. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> 使用N-十六烷烷作为模型化合物研究了Ni-zeolite催化剂（H-MFI和H-Beta）的氢代异构化/加氢裂化性能，与Ni / Asa（无定形二氧化硅 - 氧化铝）作为参考催化剂进行比较。在H-Beta的情况下，还研究了通过受控溶解引入中间渗透性的效果。结果表明，LISICALIC H-β催化剂上的Ni表示非常有趣的特性，用于从植物/藻类生产生物燃料生产中的潜在用途，或者生物量衍生的费氏杂木蜡的升级。 Ni / H-β相对于Ni / H-MFI显示出较低的活性，但显着降低气体的形成和更好的水性异构化活性。通过溶解引入中渗透性增强了活性，同时仍然保持可接受的气体形成和良好的加氢异构化性能。此外，脱气处理改善了相对于碳形成的稳定性。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16041/'>《ChemCatChem》</a> <b style="margin: 0 2px;">|</b><span>2017年第9期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=beta zeolite&option=203" rel="nofollow">beta zeolite;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=desilication&option=203" rel="nofollow">desilication;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=n-hexadecane&option=203" rel="nofollow">n-hexadecane;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hydrocracking&option=203" rel="nofollow">hydrocracking;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hydroisomerization&option=203" rel="nofollow">hydroisomerization;</a> </p> <div class="translation"> 机译：β沸石;溶解;正己烷;加氢裂化;氢异构化; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022057967.html">Effect of the Structure and Mesoporosity in Ni/Zeolite Catalysts for <i >nn ‐Hexadecane Hydroisomerisation and Hydrocracking</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> </a> <a href="/journal-foreign-16041/" target="_blank" rel="nofollow" class="tuijian_authcolor">ChemCatChem .</a> <span>2017</span><span>,第9期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：Ni /沸石催化剂中的结构和中孔率的影响 n </ i> n -Hexadecane水异构化和加氢裂化</span> </p> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/academic-journal-foreign_american-chemical-society-division-fuel-chemistry-preprints_thesis/0204110152743.html">EFFECT OF ZEOLITE MESOPOROSITY AND ACIDITY ON THE HYDROCONVERSION OF n-HEXADECANE OVER Pt/BASED CATALYSTS</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=E.F. 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href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=胡云峰&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 胡云峰</a> <span> . 2005</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/061201953534.html">微孔沸石包覆中孔沸石催化剂的制备及其在甲醇制丙烯反应中的应用</a> <b>[P]</b> . <span> 中国专利： CN103551188B </span> <span> . 2016.03.09</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120102179582.html">微孔沸石包覆中孔沸石催化剂的制备及其在甲醇制丙烯反应中的应用</a> <b>[P]</b> . <span> 中国专利： CN103551188A </span> <span> . 2014-02-05</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130445756042.html">A process for the preparation of a zeolite of the ferrierite - type which can be used as isomerization catalyst of a linear olefin to iso-olefin or as a hydrocracking - and hydroisomerisation catalyst comprises of paraffins</a> <b>[P]</b> . <span> 外国专利：  DE69801875T2 </span> <span> . 2002-06-06</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：镁碱沸石型沸石的制备方法，其可用作直链烯烃到异烯烃的异构化催化剂或加氢裂化，并且加氢异构化催化剂包含石蜡 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130501447755.html">HYDROCRACKING CATALYSTS CONTAINING RARE EARTH CONTAINING POST-MODIFIED USY ZEOLITE, METHOD FOR PREPARING HYDROCRACKING CATALYSTS, AND METHOD FOR HYDROCRACKING HYDROCARBON OIL WITH HYDROCRACKING CATALYSTS</a> <b>[P]</b> . <span> 外国专利：  US2022032273A1 </span> <span> . 2022-02-03</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：含有稀土的加氢裂化催化剂，含有后修饰的USY沸石，制备加氢裂化催化剂的方法，以及用加氢裂化催化剂加氢裂化烃油的方法 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130500894223.html">Hydrocracking catalysts containing USY and beta zeolites for hydrocarbon oil and method for hydrocracking hydrocarbon oil with hydrocracking catalysts</a> <b>[P]</b> . <span> 外国专利：  US11154845B1 </span> <span> . 2021-10-26</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：含有USY和β沸石的加氢裂化催化剂用于烃油和加氢裂化烃烃的方法用加氢裂化催化剂 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704022057967','4',7,2,1,'',this,24)" class="delivery" 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Effect of the Structure and Mesoporosity in Ni/Zeolite Catalysts for nn ‐Hexadecane Hydroisomerisation and Hydrocracking

摘要