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首页> 外文期刊>Journal of Polymer Science, Part A. Polymer Chemistry >Cyclometalated Pt complex based random terpolymers as electron acceptors for all polymer solar cells
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Cyclometalated Pt complex based random terpolymers as electron acceptors for all polymer solar cells

机译：基于环状的Pt复合物的随机萜酰基作为所有聚合物太阳能电池的电子受体

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ABSTRACT > Various molar ratios of platinum complexes were introduced into the conjugated backbone of the well‐studied poly[[ N , N ′‐bis(2‐octyldodecyl)‐naphthalene‐1,4,5,8‐bis(dicarboximide)‐2,6‐diyl]‐alt‐5,5′‐(2,2′‐bithiophene)](PNDIT2) acceptor polymer through random terpolymer approach. Terpolymers PNDIT2Ptx (x?=?1, 2 and 5) exhibited slightly higher melting point ( T <sub>m</sub> ), crystallization temperature, HOMO and LUMO energy levels than the control PNDIT2 copolymer due to the introduction of small amount of weaker electron‐withdrawing bulky rigid Pt complex instead of strong electron‐withdrawing flexible naphthalene diimide. When blended them with poly[[2,6′‐4,8‐di(5‐ethylhexylthienyl)benzo[1,2‐ b ;3,3‐ b ] dithiophene] [3‐fluoro‐2[(2‐ethylhexyl)carbonyl]thieno[3,4‐ b ]thiophenediyl]] (PTB7‐Th) in all polymer solar cells, enhanced power conversion efficiency of 4.51% (3.74%) was obtained in terpolymer PNDIT2Pt1 based device compared to 3.88% (3.24%) of the control PNDIT2 at the same inverted (conventional) device conditions. The enhancement was probably ascribed to higher hole and electron transport ability and more efficient charge separation. To the best of our knowledge, this is the first example of random terpolymer acceptors based on heavy metal complexes. ? 2017 Wiley Periodicals, Inc. J. Polym. Sci., Part A: Polym. Chem. 2018 , 56 , 105–115 </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”> <title类型=“main”>摘要</ title> >铂复合物的各种摩尔比被引入富集的聚缀合的骨干[[ n </ i>， n℃'-bis（2- octydodeCyl） - 萘-1,4,5,8-双（二​​羧酰亚胺）-2,6-二酯，5,5' - （2,2'-二甲苯烯）]（PNDIT2）受机聚合物通过随机三元共聚物方法。 Terpolymers pndit2ptx（x≤=Δ1,2和5）表现出稍高的熔点（ t </ i> <sub> m <s sub>），结晶温度，同性恋和Lumo能量水平而不是对照Pndit2共聚物由于引入少量的较弱的吸电子粗体刚性PT复合物代替强电子抽出的柔性萘二亚胺。将它们混合在聚合物中[[2,6'-4,8-​​DI（5-乙基己烯基）苯并[1,2- B </ i]; 3,3- B </ i>]二噻吩] [3-氟-2 [（2-乙基己基）羰基] Thieno [3,4- b]]噻吩（PTB7-TH）在所有聚合物太阳能电池中，增强了电力转换效率在三元共聚物PNDIT2PT1的装置中获得4.51％（3.74％），其在同一反相（常规）器件条件下的3.88％（3.24％）的对照PNDIT2。增强可能归因于更高的孔和电子传输能力和更有效的电荷分离。据我们所知，这是基于重金属配合物的随机三元共聚物受体的第一个例子。还是2017 Wiley期刊，Inc.J.Colom。 SCI。，A部分：polym。化学。 2018 </ b>， 56 </ i>，105-115 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-35621/'>《Journal of Polymer Science, Part A. Polymer Chemistry》</a> <b style="margin: 0 2px;">|</b><span>2018年第1期</span><b style="margin: 0 2px;">|</b><span>共11页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Gao Xuyu&option=202" target="_blank" rel="nofollow">Gao Xuyu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Menghan&option=202" target="_blank" rel="nofollow">Wang Menghan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cao Xudong&option=202" target="_blank" rel="nofollow">Cao Xudong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Jie&option=202" target="_blank" rel="nofollow">Yang Jie;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhong Yu&option=202" target="_blank" rel="nofollow">Zhong Yu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Zhiguo&option=202" target="_blank" rel="nofollow">Zhang Zhiguo;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Cheng&option=202" target="_blank" rel="nofollow">Li Cheng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huettner Sven&option=202" target="_blank" rel="nofollow">Huettner Sven;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tao Youtian&option=202" target="_blank" rel="nofollow">Tao Youtian;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Yongfang&option=202" target="_blank" rel="nofollow">Li Yongfang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huang Wei&option=202" target="_blank" rel="nofollow">Huang Wei;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Key Lab for Flexible Electronics and Institute of Advanced Materials Jiangsu National Synergistic Innovation Center for Advanced Materials (SICAM) Nanjing Tech University 30 South Puzhu RoadNanjing 211816 People's Republic of China;</p> <p>Key Lab for Flexible Electronics and Institute of Advanced Materials Jiangsu National Synergistic Innovation Center for Advanced Materials (SICAM) Nanjing Tech University 30 South Puzhu RoadNanjing 211816 People's Republic of China;</p> <p>Key Lab for Flexible Electronics and Institute of Advanced Materials Jiangsu National Synergistic Innovation Center for Advanced Materials (SICAM) Nanjing Tech University 30 South Puzhu RoadNanjing 211816 People's Republic of China;</p> <p>Key Lab for Flexible Electronics and Institute of Advanced Materials Jiangsu National Synergistic Innovation Center for Advanced Materials (SICAM) Nanjing Tech University 30 South Puzhu RoadNanjing 211816 People's Republic of China;</p> <p>Macromolecular Chemistry I Universit?t Bayreuth 30 Universit?tsstrBayreuth 95447 Germany;</p> <p>Beijing National Laboratory for Molecular Sciences CAS Key Laboratory of Organic Solids Institute of Chemistry Chinese Academy of SciencesBeijing 100190 People's Republic of China;</p> <p>Macromolecular Chemistry I Universit?t Bayreuth 30 Universit?tsstrBayreuth 95447 Germany;</p> <p>Macromolecular Chemistry I Universit?t Bayreuth 30 Universit?tsstrBayreuth 95447 Germany;</p> <p>Key Lab for Flexible Electronics and Institute of Advanced Materials Jiangsu National Synergistic Innovation Center for Advanced Materials (SICAM) Nanjing Tech University 30 South Puzhu RoadNanjing 211816 People's Republic of China;</p> <p>Beijing National Laboratory for Molecular Sciences CAS Key Laboratory of Organic Solids Institute of Chemistry Chinese Academy of SciencesBeijing 100190 People's Republic of China;</p> <p>Key Lab for Flexible Electronics and Institute of Advanced Materials Jiangsu National Synergistic Innovation Center for Advanced Materials (SICAM) Nanjing Tech University 30 South Puzhu RoadNanjing 211816 People's Republic of China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1184.html" title="有机化学">有机化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=conjugated polymers&option=203" rel="nofollow">conjugated polymers;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=heavy metal complex&option=203" rel="nofollow">heavy metal complex;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=non‐fullerene acceptor&option=203" rel="nofollow">non‐fullerene acceptor;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=polymer solar cells&option=203" rel="nofollow">polymer solar cells;</a> </p> <div class="translation"> 机译：共轭聚合物;重金属复合物;非富勒烯受体;聚合物太阳能电池; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704020726024.html">Cyclometalated Pt complex based random terpolymers as electron acceptors for all polymer solar cells</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Gao Xuyu&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Gao Xuyu,</a> <a 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Jalan&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Ishita Jalan,</a> <span>2021</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：具有两个不同熔环电子缺陷结构块的非共期三元共聚物受体，用于高效的全聚合物太阳能电池</span> </p> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/academic-journal-cn_acta-physico-chimica-sinica_thesis/0201271606394.html">骨架非稠合的电子受体在聚合物太阳能电池中的应用</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=章中强&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 章中强</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=张书华&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,张书华</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=刘志玺&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,刘志玺</a> <span> <a href="/journal-cn-15102/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 物理化学学报 </a> </span> <span> . 2019</span><span>,第004期</span> </span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/academic-journal-cn_detail_thesis/0201294545628.html">以C_(70)衍生物为电子受体的高效聚合物固体薄膜太阳能电池</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=王藜&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 王藜</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=徐苗&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,徐苗</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=应磊&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,应磊</a> <span> <a href="/journal-cn-56916/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 高分子学报 </a> </span> <span> . 2008</span><span>,第10期</span> </span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/academic-journal-cn_acta-physico-chimica-sinica_thesis/0201288944755.html">基于非富勒烯电子受体的半透明有机太阳能电池</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=刘柏侨&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 刘柏侨</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=许韵华&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,许韵华</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=夏冬冬&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,夏冬冬</a> <span> <a href="/journal-cn-15102/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 物理化学学报 </a> </span> <span> . 2021</span><span>,第003期</span> </span> </div> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/academic-journal-cn_journal-sichuan-university-natural-science-edition_thesis/0201270225143.html">电子受体强度对基于Thieno3,2-b thiophene的共轭聚合物电子性质的影响</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=傅杨武&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 傅杨武</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=陈明君&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,陈明君</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=周胡来&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,周胡来</a> <span> <a href="/journal-cn-4696/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 四川大学学报（自然科学版） </a> </span> <span> . 2018</span><span>,第006期</span> </span> </div> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/academic-journal-cn_spectroscopy-spectral-analysis_thesis/0201232871101.html">不同受体对 PTB7聚合物太阳能电池的性能影响的研究</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=黄迪&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 黄迪</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=徐征&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,徐征</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=赵谡玲&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,赵谡玲</a> <span> <a href="/journal-cn-11127/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 光谱学与光谱分析 </a> </span> <span> . 2016</span><span>,第008期</span> </span> </div> </li> <li> <div> <b>6. </b><a class="enjiyixqcontent" href="/academic-conference-cn_meeting-1979_thesis/02022331478.html">基于PTB7掺杂的三元有机聚合物太阳能电池的研究</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=李杨&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 李杨</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=徐征&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,徐征</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=赵谡玲&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,赵谡玲</a> <span> <a href="/conference-cn-1979/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 第十四届中国光伏大会暨2014中国国际光伏展览会 </a> <span> <span> . 2014</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/02031788462.html">基于富勒烯衍生物电子受体的聚合物太阳能电池的研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=崔颖&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 崔颖</a> <span> . 2012</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120111155519.html">聚合物太阳能电池共混活性层中的共轭小分子电子受体材料及其制备方法</a> <b>[P]</b> . <span> 中国专利： CN108659002A </span> <span> . 2018-10-16</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120112886466.html">基于噻二唑喹喔啉结构的电子受体有机太阳能电池材料及其制备方法与应用</a> <b>[P]</b> . <span> 中国专利： CN112920204A </span> <span> . 2021-06-08</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130405943722.html">Electron accepting polymer of formed random terpolymer producing method of the same and inverted type polymer solar cells comprising the same</a> <b>[P]</b> . <span> 外国专利： <!-- 韩国专利： --> KR101821971B1 </span> <span> . 2018-01-26</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：所形成的无规三元共聚物的制造方法的电子接受聚合物以及包括该方法的倒型聚合物太阳能电池 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130441257985.html">Device useful in photovoltaic cells comprises an electron donor structure comprising a conjugated polymer and an electron acceptor structure comprising a pigment complexed or adsorbed on nanotubes</a> <b>[P]</b> . <span> 外国专利： <!-- 法国专利： --> FR2849539A1 </span> <span> . 2004-07-02</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：在光伏电池中有用的装置包括包含共轭聚合物的电子给体结构和包含复合或吸附在纳米管上的颜料的电子受体结构 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130426801811.html">Solar cell e.g. tandem solar cell, has photoactive layers including regions in which mixture of electron donor materials and electron acceptor materials is provided and distinguished by compound portion of donor and acceptor materials</a> <b>[P]</b> . <span> 外国专利： <!-- 德国专利： --> DE102008050335A1 </span> <span> . 2010-04-29</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：太阳能电池串联太阳能电池，具有光敏层，该光敏层包括其中提供电子供体材料和电子受体材料的混合物并通过供体和受体材料的化合物部分来区分的区域 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704020726024','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img src="https://cdn.zhangqiaokeyan.com/img/loginclose.png" alt="关闭" 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