Enhanced nonlinear optical response of Sedoped MoS2 nanosheets for passively Q-switched fiber laser application

摘要

An enhanced nonlinear optical (NLO) performance was observed in Se-doped MoS2 nanosheets synthesized through a facile annealing process. Se-doped MoS2 nanosheets with a large saturable intensity and high modulation depth generated stable passively Q-switched fiber laser pulses at 1559 nm. In comparison with the Q-switched fiber laser utilizing the pristine MoS2 nanosheets as a saturable absorber, the passive Q-switching operation based on Se-doped MoS2 nanosheets could be conducted at a lower threshold power of 50 mW, a wider range of repetition rates from 28.97 to 130 kHz, and a higher SNR of 56 dB. More importantly, the shortest pulse duration of 1.502 mu s was realized and the output power and pulse energy reached 17.2mW and 133.07 nJ, respectively. These results indicate that tailoring the chemical composition of optical nanomaterials by introducing a dopant is a feasible method of improving the NLO response of the MoS2 nanosheets and realizing excellent ultrafast pulse generation.