<![CDATA[Beryllium-Free Nonlinear-Optical Crystals A3Ba3Li2Ga4B6O20F (A = K and Rb): Members of the Sr2Be2(BO3)2O Family with a Strong Covalent Connection]]>

Xianghe Meng; Fei Liang; Mingjun Xia; Zheshuai Lin

首页> 外文期刊>Inorganic Chemistry: A Research Journal that Includes Bioinorganic, Catalytic, Organometallic, Solid-State, and Synthetic Chemistry and Reaction Dynamics >3Ba₃Li₂Ga₄B₆O₂₀F (A = K and Rb): Members of the Sr₂Be₂(BO₃)₂O Family with a Strong Covalent Connection]]>

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3Ba₃Li₂Ga₄B₆O₂₀F (A = K and Rb): Members of the Sr₂Be₂(BO₃)₂O Family with a Strong Covalent Connection]]>

机译：<！[CDATA [铍无线 - 光学晶体A <亚> 3 BA _{3 Li _{2 ga _{4 b < 子> 6 O _{20 f（a = k和rb）：sr _{2 的成员_{2 （bo _{3 ）_{2 o系列，具有强的共价连接]]>}}}}}}}}

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机译：<！[CDATA [CDATA [基于镓的硼管，K_（3）BA_（3）LI_（2）GA_（4）B_（6）O_（20）f（ i）和rb_（3）ba_（3 ）LI_（2）GA_（4）B_（6）o_（20）f（ ii）已成功生长在M_（2）O（m = k，rb）-lif-b_（2）中生长O_（3）助焊剂。它们可以被识别为K / RB和BA的SR的元素烯项，并且来自SR_（2）BE_（2）（BO_（3））_（2）O（SBBO）的Li和Ga，其使用有毒合成和晶体生长过程中的铍氧化物也表现出结构不稳定的问题。肌肉硼酸盐结晶进入非群体对称空间组 P 6→2，用 a = 8.6398（12）？和 c = 16.827（3）？对于 i和 a = 8.7214（12）？和 c = 17.180（3）？对于 II。在结构中，基本阴离子单元是Bo_（3）三角形和GaO_（4）和LiO_（3）F Tetrahydra。这些阴离子单元通过O原子粘在一起，形成无限的延伸∞）2）[Liga_（2）B_（3）O_（12）O_（12）]〜（8-）在 AB平面上的单层。相邻的层还通过桥接O和F原子耦合到ν）2）[Li_（2）Ga_（4）B_（6）o_（20）f]〜（9-）双层。然后，相邻的双层通过GaO_（4）四德拉的O原子强烈地连接在一起，形成三维骨架，K / RB和BA原子占据网络以进行充电平衡。 I和 II具有相当大的第二次谐波产生响应，分别具有约0.7和0.5的响应，分别与KH_（2）PO_（4）一样大。此外，进行了第一原理计算以确认他们解决了SBBO中的结构不稳定问题。]]> 展开▼

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《Inorganic Chemistry: A Research Journal that Includes Bioinorganic, Catalytic, Organometallic, Solid-State, and Synthetic Chemistry and Reaction Dynamics 》 |2018年第9期| 共8页

作者
Xianghe Meng; Fei Liang; Mingjun Xia; Zheshuai Lin;
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Beijing Center for Crystal Research and Development Key Laboratory of Functional Crystals and Laser Technology Technical Institute of Physics and Chemistry Chinese Academy of Sciences Beijing 100190 China;

Beijing Center for Crystal Research and Development Key Laboratory of Functional Crystals and Laser Technology Technical Institute of Physics and Chemistry Chinese Academy of Sciences Beijing 100190 China;

Beijing Center for Crystal Research and Development Key Laboratory of Functional Crystals and Laser Technology Technical Institute of Physics and Chemistry Chinese Academy of Sciences Beijing 100190 China;

Beijing Center for Crystal Research and Development Key Laboratory of Functional Crystals and Laser Technology Technical Institute of Physics and Chemistry Chinese Academy of Sciences Beijing 100190 China;

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1. 3Ba₃Li₂Ga₄B₆O₂₀F (A = K and Rb): Members of the Sr₂Be₂(BO₃)₂O Family with a Strong Covalent Connection]]> [J] . Xianghe Meng, Fei Liang, Mingjun Xia, Inorganic Chemistry: A Research Journal that Includes Bioinorganic, Catalytic, Organometallic, Solid-State, and Synthetic Chemistry and Reaction Dynamics . 2018 ,第9期

机译：<！[CDATA [铍无线 - 光学晶体A <亚> 3 BA _{3 Li _{2 ga _{4 b < 子> 6 O _{20 f（a = k和rb）：sr _{2 的成员_{2 （bo _{3 ）_{2 o系列，具有强的共价连接]]>}}}}}}}}

2. Beryllium-Free KBBF Family of Nonlinear-Optical Crystals: AZn(2)BO(3)X(2) (A = Na, K, Rb; X = Cl, Br) [J] . Huang Qian, Liu Lijuan, Wang Xiaoyang, Inorganic Chemistry: A Research Journal that Includes Bioinorganic, Catalytic, Organometallic, Solid-State, and Synthetic Chemistry and Reaction Dynamics . 2016 ,第24期

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3Ba3Li2Ga4B6O20F (A = K and Rb): Members of the Sr2Be2(BO3)2O Family with a Strong Covalent Connection]]>

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3Ba₃Li₂Ga₄B₆O₂₀F (A = K and Rb): Members of the Sr₂Be₂(BO₃)₂O Family with a Strong Covalent Connection]]>