The influence of the magnetoelastic interaction on the magnetocaloric effect in ferrimagnetic systems: A theoretical investigation

摘要

In this work the magnetocaloric effect is theoretically investigated considering a microscopic model Hamiltonian, which describes a magnetic system formed by two sublattices of different magnetic ions coupled by exchange and magnetoelastic interactions. We analyze systematically several profiles of the ferrimagnetic arrangements that were studied earlier without the magnetoelastic interaction. The influence of changing the magnetoelastic parameters on the magnetization, isothermal entropy change and adiabatic temperature change curves are investigated. Depending on the model parameters, the magnetic system shows a first-order magnetic phase transition leading to high direct and inverse magnetocaloric effect, besides two simultaneous first-order magnetic phase transitions which were predicted. A constant ΔS_T = 0.4 J mol~(-1) K~(-1) is obtained in the simulated system in a temperature interval of 50 K, around 110 K.