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首页> 外文期刊>The Journal of Chemical Physics >Relative abundance and structure of chaotic behavior:The nonpolynomial Belousov-Zhabotinsky reaction kinetics
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Relative abundance and structure of chaotic behavior:The nonpolynomial Belousov-Zhabotinsky reaction kinetics

机译:相对丰度和混沌行为结构:非多项式Belousov-Zhabotinsky反应动力学

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摘要

We report a detailed numerical investigation of the relative abundance of periodic and chaoticoscillations in phase diagrams for the Belousov–Zhabotinsky (BZ) reaction as described by anonpolynomial, autonomous, three-variable model suggested by Gyorgyi and Field [Nature(London) 355, 808 (1992)]. The model contains 14 parameters that may be tuned to produce richdynamical scenarios. By computing the Lyapunov spectra, we find the structuring of periodic andchaotic phases of the BZ reaction to display unusual global patterns, very distinct from thoserecently found for gas and semiconductor lasers, for electric circuits, and for a few other familiarnonlinear oscillators. The unusual patterns found for the BZ reaction are surprisingly robust andindependent of the parameter explored.
机译:我们报告了有关Belousov-Zhabotinsky(BZ)反应的相图中周期和混沌振荡的相对丰度的详细数值研究,由Gyorgyi和Field [Nature(London)355,808建议的非多项式,自主,三变量模型描述(1992)]。该模型包含14个参数,可以对其进行调整以产生丰富的动态场景。通过计算Lyapunov光谱,我们发现BZ反应的周期性和混沌相的结构可以显示异常的整体模式,这与最近在气体和半导体激光器,电路以及其他一些熟悉的非线性振荡器中发现的模式非常不同。对于BZ反应发现的异常模式出奇地强大,并且与所探索的参数无关。

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