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首页> 外文期刊>Physical Review, A. Atomic, molecular, and optical physics >Role of ellipticity in high-order harmonic generation by homonuclear diatomic molecules
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Role of ellipticity in high-order harmonic generation by homonuclear diatomic molecules

机译:椭圆度在同核双原子分子高次谐波产生中的作用

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We present a theory of high-order harmonic generation by diatomic molecules exposed to an elliptically polarized laser field. This theory is based on the molecular strong-field approximation with the laser-field-dressed initial bound state and the undressed final state. The interference minima, observed for linear polarization, are blurred with the increase of the laser-field ellipticity. The nth harmonic emission rate has contributions of the components of the T -matrix element in the direction of the laser-field polarization and in the direction perpendicular to it. We analyze the destructive interference condition for this perpendicular component. Taking into account that the aligned molecules are an anisotropic medium for high-harmonic generation, we introduce elliptic dichroism as a measure of this anisotropy and discuss possibilities of its use for determining the molecular structure.
机译:我们提出了由暴露于椭圆偏振激光场的双原子分子产生高次谐波的理论。该理论基于分子强场近似,其具有激光场修饰的初始束缚态和未修饰的最终态。对于线性偏振观察到的最小干涉随着激光场椭圆率的增加而变得模糊。第n个谐波发射率在激光场偏振方向和垂直于其的方向上具有T矩阵元素的成分的贡献。我们分析了此垂直分量的相消干涉条件。考虑到排列的分子是产生高谐波的各向异性介质,我们介绍了椭圆二色性作为这种各向异性的一种度量,并讨论了其用于确定分子结构的可能性。

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