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Synthesis of cyclic 1-alkenylboronates via Zr-mediated double functionalization of alkynylboronates and sequential Ru-catalyzed ring-closing olefin metathesis

机译:通过Zr介导的炔基硼酸酯的双官能化和连续Ru催化的闭环烯烃复分解反应合成环状1-烯基硼酸酯

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摘要

Synthesis of novel cyclic 1-alkenylboronates is accomplished through the zirconium-mediated regio- and stereoselective double functionalization of 1-alkynylboronates and the subsequent ruthenium-catalyzed ring-closing metathesis (RCM). The obtained substituted cyclic 1-alkenylboronates are transformed into o-terphenyl and triphenylene derivatives.
机译:新型环状1-烯基硼酸酯的合成是通过锆介导的1-炔基硼酸酯的区域和立体选择性双官能化以及随后的钌催化的闭环复分解(RCM)完成的。将获得的取代的环状1-链烯基硼酸酯转化为邻三联苯和三亚苯基衍生物。

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