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首页> 外文期刊>The European physical journal, E. Soft matter >Reversibility and hysteresis of the sharp yielding transition of a colloidal glass under oscillatory shear
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Reversibility and hysteresis of the sharp yielding transition of a colloidal glass under oscillatory shear

机译:振荡剪切下胶态玻璃急剧屈服转变的可逆性和滞后性

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The mechanical response of glasses remains challenging to understand. Recent results indicate that the oscillatory rheology of soft glasses is accompanied by a sharp non-equilibrium transition in the microscopic dynamics. Here, we use simultaneous x-ray scattering and rheology to investigate the reversibility and hysteresis of the sharp symmetry change from anisotropic solid to isotropic liquid dynamics observed in the oscillatory shear of colloidal glasses (D. Denisov, M.T. Dang, B. Struth, A. Zaccone, P. Schall, Sci. Rep. 5 14359 (2015)). We use strain sweeps with increasing and decreasing strain amplitude to show that, in analogy with equilibrium transitions, this sharp symmetry change is reversible and exhibits systematic frequency-dependent hysteresis. Using the non-affine response formalism of amorphous solids, we show that these hysteresis effects arise from frequency-dependent non-affine structural cage rearrangements at large strain. These results consolidate the first-order-like nature of the oscillatory shear transition and quantify related hysteresis effects both via measurements and theoretical modelling.
机译:眼镜的机械响应仍然难以理解。最近的结果表明,软玻璃的振荡流变学伴随着微观动力学的急剧的非平衡转变。在这里,我们使用同时​​的X射线散射和流变学来研究在胶体玻璃的振荡剪切中观察到的从各向异性固体到各向同性液体动力学的急剧对称变化的可逆性和滞后性(D. Denisov,MT Dang,B。Struth,A Zaccone,P.Schall,Sci。Rep.5 14359(2015))。我们使用随应变振幅增大和减小的应变扫描来显示,与平衡过渡类似,这种急剧的对称变化是可逆的,并且表现出系统的频率相关滞后。使用非晶态固体的非仿射响应形式,我们显示出这些滞后效应是由大应变下依赖于频率的非仿射结构笼重新排列引起的。这些结果巩固了振荡剪切转变的一阶性质,并通过测量和理论建模来量化相关的磁滞效应。

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