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Spectral dependence of absorption photoinduced in a Bi12TiO20 crystal by 532-nm laser pulses

机译:532 nm激光脉冲在Bi12TiO20晶体中光诱导吸收的光谱依赖性

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摘要

The spectral dependences of absorption photoinduced in a pure bismuth titanium oxide crystal by 532-nm laser pulses are studied. It is shown that optical absorption in the crystal in the range from 492 to 840 urn increases with increasing exposure. The photoinduced absorption relaxes in the dark for more than 60 hours. A model of photoinduced absorption is proposed which assumes the population of two trap centres with the normal energy distribution law for the concentrations of electrons photoexcited from donors to the conduction band. This model well describes the spectral dependences of photoinduced absorption by using the average ionisation energies of the traps E-1 = 1.60 eV and E-2 = 2.57 eV. The model is used to estimate the increase in the photorefractive sensitivity of a bismuth titanium oxide crystal in the near IR region, which was earlier observed after exposing the crystal to visible radiation. It is predicted that the speed of response of dynamic holography devices based on BTO crystals exposed to green light can be increased.
机译:研究了532 nm激光脉冲在纯铋氧化钛晶体中光诱导吸收的光谱依赖性。结果表明,随着曝光量的增加,晶体在492至840 urn范围内的光吸收会增加。光吸收在黑暗中松弛超过60小时。提出了一种光致吸收模型,该模型假设两个陷阱中心的种群具有正常的能量分布定律,以供体从供体向激发带光激发的电子浓度。该模型通过使用陷阱E-1 = 1.60 eV和E-2 = 2.57 eV的平均电离能很好地描述了光诱导吸收的光谱依赖性。该模型用于估计在近红外区域中铋钛氧化物晶体的光折变敏感性的增加,这是在将晶体暴露于可见辐射后更早观察到的。预计可以提高基于暴露于绿光的BTO晶体的动态全息设备的响应速度。

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