Formation of hot-electron ensembles quasiequilibrated in momentum space by ultrafast momentum scattering of highly excited hot electrons photoinjected into the Gamma valley of GaAs

摘要

We study ultrafast scattering dynamics of hot electrons photoinjected with high excess energies in the Gamma valley of the conduction band of GaAs, using time- and angle-resolved photoemission spectroscopy and ab initio calculations. At ultrafast rates of the order of 10 fs, the packets in the Gamma valley are transformed into hot-electron ensembles (HEEs) quasiequilibrated in momentum space but not in energy space. The energy relaxation of the HEEs takes place as a whole on a longer time scale with rates dependent only on the excess energy, irrespective of the momenta of hot electrons. Both momentum scattering and energy relaxation are ruled by the electron-phonon interaction.