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Ellipticity dependence of neutral Rydberg excitation of atoms in strong laser fields

机译:强激光场中原子的中性里德堡激发的椭圆率依赖性

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Rydberg state excitation (RSE) of different atoms in elliptically polarized strong 800 nm laser fields is investigated experimentally, and the results are compared with calculations of the strong-field approximation (SFA) model and the semiclassical model. It is observed that the RSE probability declines with increasing laser ellipticity for all of the He, Ar, and Kr atoms. While the measured ellipticity dependence of He RSE is very consistent with the predictions of both the SFA and semiclassical calculations, the width of the ellipticity dependence for Ar and Kr atoms is wider than that of the SFA model but closer to the semiclassical calculations. Analysis indicates that unlike a tunneling-plus-rescattering process, the decline of the RSE yield with increasing ellipticity can be attributed to a decrease of electrons with low kinetic energy that could be captured in the Rydberg states by the Coulomb potential. It indicates that the atomic RSE process could be related to the very low or near-zero energy structure in the photoelectron spectrum in strong laser fields, which would stimulate further experimental and theoretical studies to reveal their underlying mechanisms.
机译:实验研究了椭圆偏振的800 nm强激光场中不同原子的Rydberg态激发(RSE),并将结果与​​强场近似(SFA)模型和半经典模型的计算结果进行了比较。可以看出,对于所有He,Ar和Kr原子,RSE概率都随着激光椭圆度的增加而降低。虽然He RSE的椭圆度依存性与SFA和半经典计算的预测非常吻合,但Ar和Kr原子的椭圆度依存性的宽度比SFA模型宽,但更接近于半经典计算。分析表明,与隧穿加散射过程不同,随着椭圆度的增加,RSE产率的下降可归因于动能较低的电子的减少,该动能可被库仑势捕获在里德堡态。这表明原子RSE过程可能与强激光场中光电子光谱中非常低或接近零的能量结构有关,这将刺激进一步的实验和理论研究以揭示其潜在机理。

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