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Diffusion and submonolayer island growth during hyperthermal deposition on Cu(100) and Cu(111)

机译:在Cu(100)和Cu(111)上超高温沉积过程中的扩散和亚单层岛生长

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摘要

We consider the influence of realistic island diffusion rates to homoepitaxial growth on metallic surfaces using a recently developed rate equation model which describes growth in the submonolayer regime with hyperthermal deposition. To this end, we incorporate realistic size and temperature-dependent island diffusion coefficients for the case of homoepitaxial growth on Cu(100) and Cu(111) surfaces. We demonstrate that the generic features of growth remain unaffected by the details of island diffusion, thus validating the generic scenario of high density of small islands found experimentally and theoretically for large detachment rates. However, the details of the morphological transition and scaling of the mean island size are strongly influenced by the size dependence of island diffusion. This is reflected in the scaling exponent of the mean island size, which depends on both temperature and the surface geometry.
机译:我们使用最近开发的速率方程模型来考虑现实的岛扩散速率对金属表面上同质外延生长的影响,该速率方程模型描述了具有超高温沉积的亚单层体系中的生长。为此,对于在Cu(100)和Cu(111)表面上同质外延生长的情况,我们结合了实际的尺寸和与温度相关的岛扩散系数。我们证明增长的一般特征仍然不受岛屿扩散细节的影响,从而验证了在实验上和理论上针对大脱离率发现的高密度小岛的一般情况。但是,形态变化和平均岛尺寸的定标的细节受岛扩散尺寸依赖性的影响很大。这反映在平均岛尺寸的缩放指数上,该指数取决于温度和表面几何形状。

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