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Phonon Dispersions of fcc δ-Plutonium-Gallium by Inelastic X-ray Scattering

机译:非弹性X射线散射分析fccδ-G-镓的声子色散

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We report an experimental determination of the phonon dispersion curves in a face-centered cubic (fcc) δ-plutonium-0.6 weight % gallium alloy. Several unusual features, including a large elastic anisotropy, a small-shear elastic modulus C', a Kohn-like anomaly in the T_1 branch, and a pronounced softening of the transverse modes, are found. These features can be related to the phase transitions of plutonium and to strong coupling between the lattice structure and the 5f valence instabilities. Our results also provide a critical test for theoretical treatments of highly correlated 5f electron systems as exemplified by recent dynamical mean field theory calculations for δ-plutonium.
机译:我们报告了在面心立方(fcc)δ-p-0.6重量%镓合金中声子弥散曲线的实验确定。发现了几个不同寻常的特征,包括较大的弹性各向异性,较小的剪切弹性模量C',T_1分支中的Kohn样异常以及横向模态的明显软化。这些特征可能与of的相变以及晶格结构与5f价态不稳定性之间的强耦合有关。我们的结果也为高度相关的5f电子系统的理论处理提供了关键的测试,最近的δdynamic动力学平均场理论计算证明了这一点。

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