So Close and So Different

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So Close and So Different

机译：如此亲密又如此不同

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In our solar system, the rocky planets have very distinct orbits from those of the gas giants. Carter ef al. (p. 556, published online 21 June) report on a planetary system where this pattern does not apply, posing a challenge to theories of planet formation.

机译：在我们的太阳系中，岩石行星的轨道与天然气巨星的轨道截然不同。卡特等（第556页，6月21日在线发布）报告了一个行星系统，该模式不适用，这对行星形成理论提出了挑战。

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《Science》 |2012年第6094期|p.502|共1页
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收录信息美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
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正文语种 eng
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入库时间 2022-08-18 02:53:34

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7. The thermodynamic changes that occur upon mixing five models of formamide and three models of water, including the miscibility of these model combinations itself, is studied by performing Monte Carlo computer simulations using an appropriately chosen thermodynamic cycle and the method of thermodynamic integration. The results show that the mixing of these two components is close to the ideal mixing, as both the energy and entropy of mixing turn out to be rather close to the ideal term in the entire composition range. Concerning the energy of mixing, the OPLS/AA-mod model of formamide behaves in a qualitatively different way than the other models considered. Thus, this model results in negative, while the other ones in positive energy of mixing values in combination with all three water models considered. Experimental data supports this latter behavior. Although the Helmholtz free energy of mixing always turns out to be negative in the entire composition range, the majority of the model combinations tested either show limited miscibility, or, at least, approach the miscibility limit very closely in certain compositions. Concerning both the miscibility and the energy of mixing of these model combinations, we recommend the use of the combination of the CHARMM formamide and TIP4P water models in simulations of water-formamide mixtures. [O] . Kiss, Bálint, Fábián, Balázs, Idrissi, Abdenacer, 2017

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So Close and So Different

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