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Decorrelation of the static and dynamic length scales in hard-sphere glass formers

机译:硬球玻璃成型机中静态和动态长度刻度的解相关

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摘要

We show that, in the equilibrium phase of glass-forming hard-sphere fluids in three dimensions, the staticnlength scales tentatively associated with the dynamical slowdown and the dynamical length characterizing spatialnheterogeneities in the dynamics unambiguously decorrelate. The former grow at a much slower rate than thenlatter when density increases. This observation is valid for the dynamical range that is accessible to computernsimulations, which roughly corresponds to that accessible in colloidal experiments. We also find that, in thisnsame range, no one-to-one correspondence between relaxation time and point-to-set correlation length exists.nThese results point to the coexistence of several relaxation mechanisms in the dynamically accessible regime ofnthree-dimensional hard-sphere glass formers.
机译:我们表明,在三维空间中形成玻璃的硬球流体的平衡阶段,静态长度尺度暂时与动力学减慢相关,而动态长度表征动力学中的空间异质性则明确相关。当密度增加时,前者的增长速度比后来的增长慢得多。该观察结果对于计算机模拟可访问的动态范围有效,该动态范围大致对应于胶体实验中可访问的动态范围。我们还发现,在相同范围内,弛豫时间与点对集相关长度之间不存在一一对应关系。n这些结果表明,在三维硬球体的动态可访问状态下,几种弛豫机制并存。玻璃成型器。

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  • 来源
    《PHYSICAL REVIEW E》 |2013年第4期|1-8|共8页
  • 作者单位

    Department of Chemistry Duke University Durham North Carolina 27708 USA andDepartment of Physics Duke University Durham North Carolina 27708 USA;

    LPTMC CNRS-UMR 7600 Universit´e Pierre et Marie Curie Boˆıte 121 4 Pl. Jussieu 75252 Paris c´edex 05 France;

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