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Study of radon reduction in gases for rare event search experiments

机译:用于稀有事件搜索实验的气体中ra减少量的研究

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The noble elements, argon and xenon, are frequently employed as the target and event detector for weakly interacting particles such as neutrinos and Dark Matter. For such rare processes, background radiation must be carefully minimized. Radon provides one of the most significant contaminants since it is an inevitable product of trace amounts of natural uranium. To design a purification system for reducing such contamination, the adsorption characteristics of radon in nitrogen, argon, and xenon carrier gases on various types of charcoals with different adsorbing properties and intrinsic radioactive purities have been studied in the temperature range of 190–295 K at flow rates of 0.5 and 2 standard liters per minute. Essential performance parameters for the various charcoals include the average breakthrough times (τ), dynamic adsorption coefficients (ka) and the number of theoretical stages (n). It is shown that theka-values for radon in nitrogen, argon, and xenon increase as the temperature of the charcoal traps decreases, and that they are significantly larger in nitrogen and argon than in xenon gas due to adsorption saturation effects. It is found that, unlike in xenon, the dynamic adsorption coefficients for radon in nitrogen and argon strictly obey the Arrhenius law. The experimental results strongly indicate that nitric acid etched Saratech is the best candidate among all used charcoal brands. It allows reducing total radon concentration in the LZ liquid Xe detector to meet the ultimate goal in the search for Dark Matter.
机译:稀有元素氩和氙经常用作弱相互作用粒子(如中微子和暗物质)的目标和事件检测器。对于这种罕见的过程,必须小心地最小化背景辐射。 on是最重要的污染物之一,因为它是痕量天然铀的必然产物。为了设计减少污染的净化系统,已经研究了在190–295 K的温度范围内,nitrogen在氮气,氩气和氙气载气中的吸附特性对各种类型具有不同吸附特性和固有放射性纯度的木炭的吸附特性。流量为每分钟0.5和2标准升。各种木炭的基本性能参数包括平均穿透时间(τ),动态吸附系数(ka)和理论级数(n)。结果表明,随着碳捕集阱温度的降低,氮气,氩气和氙气中the的ka值增加,并且由于吸附饱和效应,它们在氮气和氩气中的significantly值明显大于氙气中的ra。发现与氙不同,氮和氩中ra的动态吸附系数严格遵守阿伦尼乌斯定律。实验结果强烈表明,在所有使用过的木炭品牌中,硝酸蚀刻的Saratech是最佳的候选材料。它可以降低LZ液体Xe检测器中的总ra浓度,从而满足寻找暗物质的最终目标。

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