Update of the α - n Yields for Reactor Fuel Materials for the Interest of Nuclear Safeguards

摘要

The neutron yields caused by spontaneous α-decay of actinides and subsequent (α,xn) reactions were re-evaluated for the reactor fuel materials UO_2, UF_6, PuO_2 and PuF_4. For this purpose, the most recent reference data for decay parameters, α-particle stopping powers and (α,xn) cross sections were collected, analysed and used in calculations. The input data and elaborated code were validated against available thick target neutron yields in pure and compound materials measured at accelerators or with radioactive sources. This paper provides the specific neutron yields and their uncertainties resultant from a-decay of actinides ~(241)Am, ~(249)Bk, ~(252)Cf, ~(242,244)Cm, ~(237)Np, ~(238-242)Pu, ~(232)Th and ~(232-236,238)U in oxide and fluoride compounds. The obtained results are an update of previous reference tables issued by the Los Alamos National Laboratory in 1991 which were used for the safeguarding of radioactive materials by passive non-destructive techniques. The comparison of the updated values with previous ones shows an agreement within one estimated uncertainty (≈10%) for oxides, and deviations of up to 50% for fluorides.