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Preparation and characterization of Pt-TiO_2-SiO_2 mesoporous materials and visible-light photocatalytic performance

机译:Pt-TiO_2-SiO_2介孔材料的制备,表征及可见光催化性能

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摘要

TiO_2-SiO_2 metal oxide materials with a mesostructure have been prepared by a novel method in which hydrolysis and condensation of titanium tetraisopropoxide (TTIP) and tetraethoxysilane (TEOS) were controlled by the pH change of acidic solution. The Pt-modified TiO_2-SiO_2 catalysts were synthesized by the photo-reduction method. The resulting materials showed a high photocatalytic activity for the photodegradation of methyl orange in the visible-light range. A reaction mechanism was proposed and discussed.
机译:采用新型方法制备了介孔结构的TiO_2-SiO_2金属氧化物材料,该方法通过控制酸性溶液的pH值来控制四异丙氧基钛(TTIP)和四乙氧基硅烷(TEOS)的水解和缩合。采用光还原法合成了Pt改性的TiO_2-SiO_2催化剂。所得材料对可见光范围内的甲基橙的光降解表现出高的光催化活性。提出并讨论了反应机理。

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