Evaluating remediation of radionuclide contaminated forest near Iwaki, Japan, using radiometric methods

摘要

Radiometric surveys have been conducted in support of a project investigating the potential of biofuel power generation coupled with remediation of forests contaminated with radionuclides following the Fukushima Daiichi accident. Surveys conducted in 2013 and 2014 were used to determine the distribution and time dependence of radionuclides in a cedar plantation and adjacent deciduous forestry subject to downslope radionuclide migration, and a test area where litter removal was conducted. The radiocaesium results confirmed enhanced deposition levels in the evergreen areas compared" with adjacent areas" of deciduous forestry, implying significant differences in depositional processes during the initial interception period in 2011. Surveys were conducted both with and without a collimator on both occasions, which modified the angular response of the detector to separate radiation signals from above and below the detector. The combined data have been used to define the influence of radionuclides in the forest canopy on dose rate at 1 m, indicating that, in evergreen areas, the activity retained within the canopy even by 2013 contributed less than 5% of ground level dose rate. The time dependent changes observed allow the effect of remediation by litter removal in reducing radionuclide inventories and dose rates to be appraised relative natural redistribution processes on adjacent control areas. A 15 x 45 m area of cedar forest was remediated in September 2013. The work involved five people in a total of 160 person hours. It incurred a total dose of 40-50 mu Sv, and generated 2.1 t of waste comprising forest litter and understory. Average dose rates were reduced from 031 mu Sv h(-1) to 0.22 mu Sv h(-1), with nuclide specific analyses indicating removal of 30 +/- 3% of the local radiocaesium inventory. This compares with annual removal rates of 10-15% where radionuclide migration down -slope over ranges of 10-50 m could be observed within adjacent areas. Local increases were also observed in areas identified as sinks. The results confirm the utility of time -series, collimated, radiometric survey methods to account for the- distribution"and changes in radionuclide inventory within contaminatedlorests. The data on litter removal imply that significant activity transfer from canopy to soil had taken place, and provide benchmark results against which such remediation actions can be appraised. (C) 2016 Elsevier Ltd. All rights reserved.