首页> 外文期刊>International journal of hydrogen energy >Highly performed non-humidification membrane electrode assembly prepared with binary RuO_2-SiO_2 oxide supported Pt catalysts as anode
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Highly performed non-humidification membrane electrode assembly prepared with binary RuO_2-SiO_2 oxide supported Pt catalysts as anode

机译:以二元RuO_2-SiO_2氧化物负载的Pt催化剂为阳极制备的高性能非增湿膜电极组件

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摘要

The use of non-humidification membrane electrode assembly (MEA) greatly reduces system cost and sophistication of polymer electrolyte membrane fuel cells (PEMFCs). An attempt to develop non-humidifying MEA without external gas humidification is made in this work using a home-made multi-functional Pt/RuO_2-SiO_2/C as the anode catalyst. Compared with MEA with Pt/SiO_2/C or Pt/C anodes, the better wettability of MEA with Pt/ RuO_2-SiO_2/C is confirmed by contact angle measurements. Single fuel cell tests with and without external gas humidification indicate that MEA with Pt/RuO_2-SiO_2/C (3 wt.% RuO_2) displays the best performance. Under non-humidification operation conditions, the MEA with Pt/RuO_2-SiC>2/C discharges at 0.6 V for 48 h with only a slight current density decay.
机译:非加湿膜电极组件(MEA)的使用大大降低了系统成本,并降低了聚合物电解质膜燃料电池(PEMFC)的复杂性。在这项工作中,尝试使用自制的多功能Pt / RuO_2-SiO_2 / C作为阳极催化剂,开发了一种无需外部气体加湿的非加湿MEA。与具有Pt / SiO_2 / C或Pt / C阳极的MEA相比,通过接触角测量可以确认MEA与Pt / RuO_2-SiO_2 / C的润湿性更好。具有和不具有外部气体加湿的单燃料电池测试表明,具有Pt / RuO_2-SiO_2 / C(3 wt。%RuO_2)的MEA显示出最佳性能。在非加湿操作条件下,具有Pt / RuO_2-SiC> 2 / C的MEA在0.6 V的电压下放电48小时,电流密度仅略有衰减。

著录项

  • 来源
    《International journal of hydrogen energy》 |2012年第17期|p.13103-13109|共7页
  • 作者单位

    School of Chemistry and Chemical Engineering, South China University of Technology, Guangzhou 510641, China,Guangdong Key Lab for Fuel Cell Technology & Key Lab of Enhanced Heat Transfer and Energy Conservation, South China University of Technology, Ministry of Education, Guangzhou 510641, China;

    School of Chemistry and Chemical Engineering, South China University of Technology, Guangzhou 510641, China,Guangdong Key Lab for Fuel Cell Technology & Key Lab of Enhanced Heat Transfer and Energy Conservation, South China University of Technology, Ministry of Education, Guangzhou 510641, China;

    School of Chemistry and Chemical Engineering, South China University of Technology, Guangzhou 510641, China,Guangdong Key Lab for Fuel Cell Technology & Key Lab of Enhanced Heat Transfer and Energy Conservation, South China University of Technology, Ministry of Education, Guangzhou 510641, China;

    School of Chemistry and Chemical Engineering, South China University of Technology, Guangzhou 510641, China,Guangdong Key Lab for Fuel Cell Technology & Key Lab of Enhanced Heat Transfer and Energy Conservation, South China University of Technology, Ministry of Education, Guangzhou 510641, China,School of Chemistry and Chemical Engineering, South China University of Technology, 381 Wushan Road,Tianhe District, Guangzhou 510641, China;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    non-humidification; membrane electrode assembly; anode catalyst; polymer electrolyte membrane fuel; cells;

    机译:非加湿膜电极组件阳极催化剂;聚合物电解质膜燃料;细胞;
  • 入库时间 2022-08-18 00:28:26

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