Aerosol-induced direct radiative forcing effects on terrestrial ecosystem carbon fluxes over China

摘要

Atmospheric aerosols can change vegetation photosynthesis through the effects of aerosols on radiation, which will affect the peak carbon dioxide emissions and carbon neutrality at global scales. In this study, we quantify the aerosol-induced direct radiation forcing (ADRF) in China from 2001 to 2014 based on the radiation flux simulation used by the Fu-Liou radiation transfer model under with-aerosols and no-aerosols scenarios. Using the radiation simulation results, we modify the atmospheric forcing datasets to drive Community Land Model 4.5 (CLM4.5) to gain the changes in carbon fluxes in China caused by ADRF. The results show that these two models are accurate in estimating radiation (R~2 = 0.78-0.88) and carbon fluxes (R~2 = 0.73-0.75) in China. High levels of ADRFs were captured in China, especially with increasing diffuse fraction, resulting in the diffusing fertilization effect occurring in most areas of China. The ADRF can increase cumulative gross primary productivity (GPP) and total ecosystem respiration (ER) by 3.20 gC m~(-2) and 5.13 gC m~(-2) per year, respectively. From 2001 to 2014, the diffusing fertilization effects experienced trends of increasing first and then decreasing. However, ADRFs in some regions of China show negative effects on carbon fluxes due to vulnerable vegetation functional types and high aerosol loading. The ADRF will also enable soil temperature decreases and volumetric soil water increases, which is closely related to changes in carbon fluxes. Meanwhile, due to changes in soil water and heat conditions, N_2O and CH_4 production will also be disturbed, and ADRF increases the global warming potential (GWP) for both greenhouse gases. This phenomenon indicated that atmospheric aerosol pollution control is far-reaching significance for peaking carbon dioxide emissions before 2030.