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ASPEN plus modelling of air–steam gasification of biomass with sorbent enabled CO2 capture

机译:ASPEN加上具有吸附剂的CO 2 捕获 的生物质的空气-蒸汽气化的建模

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Abstract The work deals with the modelling and simulation of carbon dioxide capture in air–steam gasification of saw dust using {ASPEN} Plus process simulator. The proposed quasi-steady state model incorporates pyrolysis, tar cracking and char conversion using existing experimental data. Prediction accuracy of the developed model is validated by comparing with available experimental results. Effects of CaO addition in air–steam gasification are analysed through key operating parameters such as gasification temperature, equivalence ratio, steam to biomass ratio and gasification efficiency. Maximum {H2} mole fraction of 31.17% is obtained at a temperature of 900?K, equivalence ratio of 0.25, and steam to biomass ratio and sorbent to biomass ratio of unity. The {H2} and {CO2} mole fractions are found to be increased and decreased by 28.10% and 42.6%, respectively, when compared with the corresponding non- sorbent case.
机译:摘要这项工作使用{ASPEN} Plus工艺模拟器对锯末的空气-蒸汽气化过程中二氧化碳捕集进行建模和模拟。拟议的准稳态模型结合了热解,焦油裂化和使用现有实验数据进行的焦炭转化。通过与可用的实验结果进行比较,验证了所开发模型的预测准确性。通过关键操作参数,例如气化温度,当量比,蒸汽与生物质之比和气化效率,分析了CaO在空气-蒸汽气化中的影响。在900?K,当量比为0.25,蒸汽与生物质比和吸附剂与生物质比为1的条件下,最大{H2}摩尔分数为31.17%。与相应的非吸附剂情况相比,发现{H 2}和{CO 2}摩尔分数分别增加和减少了28.10%和42.6%。

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